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Molecular Design Strategy of Organic Thermally Activated Delayed Fluorescence Emitters
Abstract
Recently, organic thermally activated delayed fluorescence (TADF) emitters have attracted a great deal of attention because they can theoretically realize 100% internal quantum efficiency. Many TADF emitters have been developed since the first demonstration of close to 20% external quantum efficiency in the devices. Recently developed TADF emitters demonstrated close to 37% external quantum efficiency in blue, above 30% external quantum efficiency in green, and close to 18% external quantum efficiency in red devices. Therefore, TADF organic light-emitting diodes could potentially be substituted for high-efficiency phosphorescent organic light-emitting diodes. In this work, we reviewed molecular design strategies of organic-based TADF emitters by classifying them into several categories depending on the material parameters required for the TADF emitters. In addition, we proposed a future development direction of TADF emitters to make them competitive with phosphorescent emitters.
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Cited by
All-organic thermally activated delayed fluorescence materials for organic light-emitting diodes
Liu, Y., Li, C., Ren, Z., Yan, S., & Bryce, M. R. (2018) · Nature Reviews Materials · doi:10.1038/natrevmats.2018.20 · Cited by 1,644
Xu, Y., Cheng, Z., Li, Z., Liang, B., Wang, J., Wei, J., Zhang, Z., & Wang, Y. (2020) · Advanced Optical Materials · doi:10.1002/adom.201902142 · Cited by 513
Liang, X., Yan, Z., Han, H., Wu, Z., Zheng, Y., Meng, H., Zuo, J., & Huang, W. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201806323 · Cited by 426
Yuan, Y., Tang, X., Du, X., Hu, Y., Yu, Y., Jiang, Z., Liao, L., & Lee, S. (2019) · Advanced Optical Materials · doi:10.1002/adom.201801536 · Cited by 404
Wu, X., Ni, S., Wang, C.-H., Zhu, W., & Chou, P.-T. (2025) · Chemical Reviews · doi:10.1021/acs.chemrev.5c00021 · Cited by 325
Metadata
- Authors
- Im, Y., Kim, M., Cho, Y. J., Seo, J.-A., Yook, K. S., & Lee, J. Y.
- Venue
- Chemistry of Materials
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-02-22
- Volume
- 29
- Issue
- 5
- Pages
- 1946-1963
- ISSN
- 0897-4756 (ISSN-L)
- 1520-5002
- OpenAlex
- W2587466492
- Cited by
- 1,058
- References
- 0
- FWCI
- 40.84
- Type
- journal article
- Language
- en
- Open access
- closed
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- Im, Y., Kim, M., Cho, Y. J., Seo, J.-A., Yook, K. S., & Lee, J. Y. (2017). Molecular Design Strategy of Organic Thermally Activated Delayed Fluorescence Emitters. Chemistry of Materials. https://doi.org/10.1021/acs.chemmater.6b05324
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