The DOI matches its Crossref record; 43 of the 43 references it cites were found in a registry or an index.
Thermoelectric Properties of Two-Dimensional Molybdenum-Based MXenes
Abstract
MXenes are an interesting class of 2D materials consisting of transition metal carbides and nitrides, which are currently a subject of extensive studies. Although there have been theoretical calculations estimating the thermoelectric properties of MXenes, no experimental measurements have been reported so far. In this report, three compositions of Mo-based MXenes (Mo 2 CT x, Mo 2 TiC 2 T x, and Mo 2 Ti 2 C 3 T x ) have been synthesized and processed into free-standing binder-free papers by vacuum-assisted filtration, and their electrical and thermoelectric properties are measured. Upon heating to 800 K, these MXene papers exhibit high conductivity and n-type Seebeck coefficient. The thermoelectric power reaches 3.09 × 10 –4 W m –1 K –2 at 803 K for the Mo 2 TiC 2 T x MXene. While the thermoelectric properties of MXenes do not reach that of the best materials, they exceed their parent ternary and quaternary layered carbides. Mo 2 TiC 2 T x shows the highest electrical conductivity in combination with the largest Seebeck coefficient of the three 2D materials studied.
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Cites
Two‐Dimensional Nanocrystals Produced by Exfoliation of Ti3AlC2
Naguib, M., Kurtoglu, M., Presser, V., Lu, J., Niu, J., Heon, M., Hultman, L., Gogotsi, Y., & Barsoum, M. W. (2011) · Advanced Materials · doi:10.1002/adma.201102306 · Cited by 11,855
Self-citation2D metal carbides and nitrides (MXenes) for energy storage
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Self-citationConductive two-dimensional titanium carbide ‘clay’ with high volumetric capacitance
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Self-citationElectromagnetic interference shielding with 2D transition metal carbides (MXenes)
Shahzad, F., Alhabeb, M., Hatter, C. B., Anasori, B., Man Hong, S., Koo, C. M., & Gogotsi, Y. (2016) · Science · doi:10.1126/science.aag2421 · Cited by 5,201
Self-citationCation Intercalation and High Volumetric Capacitance of Two-Dimensional Titanium Carbide
Lukatskaya, M. R., Mashtalir, O., Ren, C. E., Dall’Agnese, Y., Rozier, P., Taberna, P. L., Naguib, M., Simon, P., Barsoum, M. W., & Gogotsi, Y. (2013) · Science · doi:10.1126/science.1241488 · Cited by 4,320
Self-citationExperimental Realization of a Three-Dimensional Topological Insulator, Bi 2 Te 3
Chen, Y. L., Analytis, J. G., Chu, J.-H., Liu, Z. K., Mo, S.-K., Qi, X. L., Zhang, H. J., Lu, D. H., Dai, X., Fang, Z., et al. (2009) · Science · doi:10.1126/science.1173034 · Cited by 3,585
Flexible and conductive MXene films and nanocomposites with high capacitance
Ling, Z., Ren, C. E., Zhao, M.-Q., Yang, J., Giammarco, J. M., Qiu, J., Barsoum, M. W., & Gogotsi, Y. (2014) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.1414215111 · Cited by 2,274
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New Two-Dimensional Niobium and Vanadium Carbides as Promising Materials for Li-Ion Batteries
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Self-citationTwo-Dimensional, Ordered, Double Transition Metals Carbides (MXenes)
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Cited by
Jiang, X., Kuklin, A. V., Baev, A., Ge, Y., Ågren, H., Zhang, H., & Prasad, P. N. (2020) · Physics Reports · doi:10.1016/j.physrep.2019.12.006 · Cited by 914
Recent Advances in Oxidation Stable Chemistry of 2D MXenes
Cao, F., Zhang, Y., Wang, H., Khan, K., Tareen, A. K., Qian, W., Zhang, H., & Ågren, H. (2022) · Advanced Materials · doi:10.1002/adma.202107554 · Cited by 648
MXenes: An Introduction of Their Synthesis, Select Properties, and Applications
Verger, L., Natu, V., Carey, M., & Barsoum, M. W. (2019) · Trends in Chemistry · doi:10.1016/j.trechm.2019.04.006 · Cited by 499
Recent Progress of Two-Dimensional Thermoelectric Materials
Li, D., Gong, Y., Chen, Y., Lin, J., Khan, Q., Zhang, Y., Li, Y., Zhang, H., & Xie, H. (2020) · Nano-Micro Letters · doi:10.1007/s40820-020-0374-x · Cited by 429
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Metadata
- Authors
- Kim, H., Anasori, B., Gogotsi, Y., & Alshareef, H. N.
- Venue
- Chemistry of Materials
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-07-17
- Volume
- 29
- Issue
- 15
- Pages
- 6472-6479
- ISSN
- 0897-4756 (ISSN-L)
- 1520-5002
- OpenAlex
- W2732829215
- Cited by
- 448
- References
- 43
- FWCI
- 10.39
- Type
- journal article
- Language
- en
- Open access
- closed
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