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Enhanced Raman Scattering with Dielectrics
Abstract
Dielectrics represent a new frontier for surface-enhanced Raman scattering. They can serve as either a complement or an alternative to conventional, metal-based SERS, offering key advantages in terms of low invasiveness, reproducibility, versatility, and recyclability. In comparison to metals, dielectric systems and, in particular, semiconductors are characterized by a much greater variety of parameters and properties that can be tailored to achieve enhanced Raman scattering or related effects. Light-trapping and subwavelength-focusing capabilities, morphology-dependent resonances, control of band gap and stoichiometry, size-dependent plasmons and excitons, and charge transfer from semiconductors to molecules and vice versa are a few examples of the manifold opportunities associated with the use of semiconductors as SERS-active materials. This review provides a broad analysis of SERS with dielectrics, encompassing different optical phenomena at the basis of the Raman scattering enhancement and introducing future challenges for light harvesting, vibrational spectroscopy, imaging, and sensing.
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Beiträge zur Optik trüber Medien, speziell kolloidaler Metallösungen
Mie, G. (1908) · Annalen der Physik · doi:10.1002/andp.19083300302 · Cited by 11,537
Surface raman spectroelectrochemistry
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Non-plasmonic nanoantennas for surface enhanced spectroscopies with ultra-low heat conversion
Caldarola, M., Albella, P., Cortés, E., Rahmani, M., Roschuk, T., Grinblat, G., Oulton, R. F., Bragas, A. V., & Maier, S. A. (2015) · Nature Communications · doi:10.1038/ncomms8915 · Cited by 520
Cited by
Surface-enhanced Raman spectroscopy: benefits, trade-offs and future developments
Pérez-Jiménez, A. I., Lyu, D., Lu, Z., Liu, G., & Ren, B. (2020) · Chemical Science · doi:10.1039/d0sc00809e · Cited by 912
Semiconductor SERS enhancement enabled by oxygen incorporation
Zheng, Z., Cong, S., Gong, W., Xuan, J., Li, G., Lu, W., Geng, F., & Zhao, Z. (2017) · Nature Communications · doi:10.1038/s41467-017-02166-z · Cited by 452
Dielectric Resonant Metaphotonics
Koshelev, K., & Kivshar, Y. (2021) · ACS Photonics · doi:10.1021/acsphotonics.0c01315 · Cited by 382
Surface-enhanced Raman spectroscopy: a half-century historical perspective
Yi, J., You, E.-M., Hu, R., Wu, D.-Y., Liu, G.-K., Yang, Z.-L., Zhang, H., Gu, Y., Wang, Y.-H., Wang, X., et al. (2025) · Chemical Society Reviews · doi:10.1039/d4cs00883a · Cited by 382
A Novel Ultra‐Sensitive Semiconductor SERS Substrate Boosted by the Coupled Resonance Effect
Yang, L., Peng, Y., Yang, Y., Liu, J., Huang, H., Yu, B., Zhao, J., Lu, Y., Huang, Z., Li, Z., et al. (2019) · Advanced Science · doi:10.1002/advs.201900310 · Cited by 298
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Metadata
- Authors
- Alessandri, I., & Lombardi, J. R.
- Venue
- Chemical Reviews
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-10-14
- Volume
- 116
- Issue
- 24
- Pages
- 14921-14981
- ISSN
- 0009-2665 (ISSN-L)
- 1520-6890
- OpenAlex
- W2530188073
- Cited by
- 655
- References
- 4
- FWCI
- 1.52
- Type
- journal article
- Language
- en
- Open access
- closed
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