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Development of Redox-Active Flow Electrodes for High-Performance Capacitive Deionization
Open accessAbstract
An innovative flow electrode comprising redox-active quinones to enhance the effectiveness of water desalination using flow-electrode capacitive deionization (FCDI) is described in this study. The results show that, in addition to carbon particle contact, the presence of the aqueous hydroquinone (H 2 Q)/benzoquinone (Q) couple in a flowing suspension of carbon particles enhances charge transfer significantly as a result of reversible redox reactions of H 2 Q/Q. Ion migration through the micropores of the flow electrodes was facilitated in particular with the desalination rate significantly enhanced. The cycling behavior of the quinoid mediators in the anode flow electrode demonstrated a relatively high stability at the low pH induced, suggesting that the mediator would be suitable for long-term operation.
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Cites
Anderson, M. A., Cudero, A. L., & Palma, J. (2010) · Electrochimica Acta · doi:10.1016/j.electacta.2010.02.012 · Cited by 943
Desalination via a New Membrane Capacitive Deionization Process Utilizing Flow-Electrodes
Jeon, S.-I., Park, H.-R., Yeo, J.-G., Yang, S., Cho, C. H., Han, M. H., & Kim, D. K. (2013) · Energy & Environmental Science · doi:10.1039/c3ee24443a · Cited by 727
Cited by
Zhang, C., Ma, J., Wu, L., Sun, J., Wang, L., Li, T., & Waite, T. D. (2021) · Environmental Science & Technology · doi:10.1021/acs.est.0c06552 · Cited by 323
Self-citationEnergy Efficiency of Capacitive Deionization
Wang, L., Dykstra, J. E., & Lin, S. (2019) · Environmental Science & Technology · doi:10.1021/acs.est.8b04858 · Cited by 292
Review of Concepts and Applications of Electrochemical Ion Separation (EIONS) Process
Yoon, H., Lee, J., Kim, S., & Yoon, J. (2019) · Separation and Purification Technology · doi:10.1016/j.seppur.2018.12.071 · Cited by 133
Metadata
- Authors
- Ma, J., He, D., Tang, W., Kovalsky, P., He, C., Zhang, C., & Waite, T. D.
- Venue
- Environmental Science & Technology
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-11-30
- Volume
- 50
- Issue
- 24
- Pages
- 13495-13501
- ISSN
- 0013-936X (ISSN-L)
- 1520-5851
- OpenAlex
- W2550284290
- Cited by
- 166
- References
- 2
- FWCI
- 6.08
- Type
- journal article
- Language
- en
- Open access
- green
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