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CH3NH3PbCl3 Single Crystals: Inverse Temperature Crystallization and Visible-Blind UV-Photodetector
Open accessAbstract
Single crystals of hybrid perovskites have shown remarkably improved physical properties compared to their polycrystalline film counterparts, underscoring their importance in the further development of advanced semiconductor devices. Here we present a new method of growing sizable CH3NH3PbCl3 single crystals based on the retrograde solubility behavior of hybrid perovskites. We show, for the first time, the energy band structure, charge recombination, and transport properties of CH3NH3PbCl3 single crystals. These crystals exhibit trap-state density, charge carrier concentration, mobility, and diffusion length comparable with the best quality crystals of methylammonium lead iodide or bromide perovskites reported so far. The high quality of the crystal along with its suitable optical band gap enabled us to build an efficient visible-blind UV-photodetector, demonstrating its potential in optoelectronic applications.
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Kim, H.-S., Lee, C.-R., Im, J.-H., Lee, K.-B., Moehl, T., Marchioro, A., Moon, S.-J., Humphry-Baker, R., Yum, J.-H., Moser, J. E., et al. (2012) · Scientific Reports · doi:10.1038/srep00591 · Cited by 8,092
Cited by
Triple-halide wide–band gap perovskites with suppressed phase segregation for efficient tandems
Xu, J., Boyd, C. C., Yu, Z. J., Palmstrom, A. F., Witter, D. J., Larson, B. W., France, R. M., Werner, J., Harvey, S. P., Wolf, E. J., et al. (2020) · Science · doi:10.1126/science.aaz5074 · Cited by 1,080
Ahmadi, M., Wu, T., & Hu, B. (2017) · Advanced Materials · doi:10.1002/adma.201605242 · Cited by 820
Self-citationPan, J., Sarmah, S. P., Murali, B., Dursun, I., Peng, W., Parida, M. R., Liu, J., Sinatra, L., Alyami, N., Zhao, C., et al. (2015) · The Journal of Physical Chemistry Letters · doi:10.1021/acs.jpclett.5b02460 · Cited by 527
Self-citationSaidaminov, M. I., Abdelhady, A. L., Maculan, G., & Bakr, O. M. (2015) · Chemical Communications · doi:10.1039/c5cc06916e · Cited by 468
Self-citationHeterovalent Dopant Incorporation for Bandgap and Type Engineering of Perovskite Crystals
Abdelhady, A. L., Saidaminov, M. I., Murali, B., Adinolfi, V., Voznyy, O., Katsiev, K., Alarousu, E., Comin, R., Dursun, I., Sinatra, L., et al. (2016) · The Journal of Physical Chemistry Letters · doi:10.1021/acs.jpclett.5b02681 · Cited by 409
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Metadata
- Authors
- Maculan, G., Sheikh, A. D., Abdelhady, A. L., Saidaminov, M. I., Haque, M. A., Murali, B., Alarousu, E., Mohammed, O. F., Wu, T., & Bakr, O. M.
- Venue
- The Journal of Physical Chemistry Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-09-17
- Volume
- 6
- Issue
- 19
- Pages
- 3781-3786
- ISSN
- 1948-7185 (ISSN-L)
- OpenAlex
- W1443040875
- Cited by
- 791
- References
- 1
- FWCI
- 34.16
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Maculan, G., Sheikh, A. D., Abdelhady, A. L., Saidaminov, M. I., Haque, M. A., Murali, B., Alarousu, E., Mohammed, O. F., Wu, T., & Bakr, O. M. (2015). CH3NH3PbCl3 Single Crystals: Inverse Temperature Crystallization and Visible-Blind UV-Photodetector. The Journal of Physical Chemistry Letters. https://doi.org/10.1021/acs.jpclett.5b01666
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