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Cited by 1,028

The DOI matches its Crossref record; 6 of the 6 references it cites were found in a registry or an index.

Electrode–Electrolyte Interface in Li-Ion Batteries: Current Understanding and New Insights

Gauthier, Magali, Carney, Thomas J., Grimaud, Alexis, Giordano, Livia, Pour, Nir, Chang, Hao-Hsun, Fenning, David P., Lux, Simon F., Paschos, Odysseas, Bauer, Christoph, Maglia, Filippo, Lupart, Saskia, Lamp, Peter, Shao-Horn, Yang·2015·The Journal of Physical Chemistry Letters

Abstract

Understanding reactions at the electrode/electrolyte interface (EEI) is essential to developing strategies to enhance cycle life and safety of lithium batteries. Despite research in the past four decades, there is still limited understanding by what means different components are formed at the EEI and how they influence EEI layer properties. We review findings used to establish the well-known mosaic structure model for the EEI (often referred to as solid electrolyte interphase or SEI) on negative electrodes including lithium, graphite, tin, and silicon. Much less understanding exists for EEI layers for positive electrodes. High-capacity Li-rich layered oxides yLi2-xMnO3·(1-y)Li1-xMO2, which can generate highly reactive species toward the electrolyte via oxygen anion redox, highlight the critical need to understand reactions with the electrolyte and EEI layers for advanced positive electrodes. Recent advances in in situ characterization of well-defined electrode surfaces can provide mechanistic insights and strategies to tailor EEI layer composition and properties.

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Metadata

Authors
Gauthier, M., Carney, T. J., Grimaud, A., Giordano, L., Pour, N., Chang, H.-H., Fenning, D. P., Lux, S. F., Paschos, O., Bauer, C., Maglia, F., Lupart, S., Lamp, P., & Shao-Horn, Y.
Venue
The Journal of Physical Chemistry Letters
Published
2015-11-11
Volume
6
Issue
22
Pages
4653-4672
ISSN
1948-7185 (ISSN-L)
OpenAlex
W2301871377
Cited by
1,028
References
6
FWCI
37.69
Type
journal article
Language
en
Open access
closed

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CoChat. (2026). Citation check: Electrode–Electrolyte Interface in Li-Ion Batteries: Current Understanding and New Insights. https://app.cochat.ai/papers/10.1021/acs.jpclett.5b01727
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Gauthier, M., Carney, T. J., Grimaud, A., Giordano, L., Pour, N., Chang, H.-H., Fenning, D. P., Lux, S. F., Paschos, O., Bauer, C., Maglia, F., Lupart, S., Lamp, P., & Shao-Horn, Y. (2015). Electrode–Electrolyte Interface in Li-Ion Batteries: Current Understanding and New Insights. The Journal of Physical Chemistry Letters. https://doi.org/10.1021/acs.jpclett.5b01727

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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).

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