Advanced Model for Solid Electrolyte Interphase Electrodes in Liquid and Polymer Electrolytes
Open accessAbstract
Recent studies show that the SEI on lithium and on anodes in liquid nonaqueous solutions consists of many different materials including , LiF, LiCl, , alkoxides, and nonconducting polymers. The equivalent circuit for such a mosaic‐type SEI electrode is extremely complex. It is shown that near room temperature the grain‐boundary resistance ( R gb ) for polyparticle solid electrolytes is larger than the bulk ionic resistance. Up to now, all models of SEI electrodes ignored the contribution of R gb to the overall SEI resistance. We show here that this neglect has no justification. On the basis of recent results, we propose here for SEI electrodes equivalent circuits which take into account the contribution of grain‐boundary and other interfacial impedance terms. This model accounts for a variety of different types of Nyquist plots reported for lithium and electrodes in liquid nonaqueous and polymer electrolytes.
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The SEI formed in standard electrolyte resembles the mosaic structure predicted by Peled et al., which describes the SEI as a heterogeneous distribution of inorganic and organic components.
“The SEI formed in this standard electrolyte resembles the mosaic structure predicted by Peled et al. [166], who described the SEI as a heterogeneous distribution of inorganic and organic components.”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [166]
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- Authors
- Peled, E., Golodnitsky, D., & Ardel, G.
- Affiliations
- Tel Aviv University (IL)
- Venue
- Journal of The Electrochemical Society
- Publisher
- The Electrochemical Society
- Published
- 1997-08-01
- Volume
- 144
- Issue
- 8
- Pages
- L208-L210
- ISSN
- 0013-4651 (ISSN-L)
- 1945-7111
- OpenAlex
- W2037447290
- Cited by
- 1,205
- References
- 0
- Citations by year
- 2026: 86 · 2025: 96 · 2024: 110 · 2023: 119 · 2022: 99 · 2021: 129 · 2020: 107 · 2019: 88 · 2018: 65 · 2017: 51 · 2016: 32 · 2015: 37 · 2014: 37 · 2013: 21 · 2012: 25
- FWCI
- 4.51
- Type
- journal article
- Language
- en
- Open access
- bronze
- doi.org
- Licence
- Locations
- Journal of The Electrochemical Society (publishedVersion)
- Funders
- Tel Aviv University
- Ministry of Defense
- U.S. Air Force
- Topics
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Advanced Battery Materials and Technologies
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Advancements in Battery Materials
- Physical Sciences › Engineering › Automotive Engineering › Advanced Battery Technologies Research
- Keywords
- solid electrolyte interphase, grain boundary resistance, interfacial impedance, lithium metal anode, lithium-ion batteries, polymer electrolytes, Nyquist plot, lithium fluoride
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