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Charge- and Size-Selective Ion Sieving Through Ti3C2Tx MXene Membranes
Open accessAbstract
Nanometer-thin sheets of 2D Ti3C2Tx (MXene) have been assembled into freestanding or supported membranes for the charge- and size-selective rejection of ions and molecules. MXene membranes with controllable thicknesses ranging from hundreds of nanometers to several micrometers exhibited flexibility, high mechanical strength, hydrophilic surfaces, and electrical conductivity that render them promising for separation applications. Micrometer-thick MXene membranes demonstrated ultrafast water flux of 37.4 L/(Bar·h·m(2)) and differential sieving of salts depending on both the hydration radius and charge of the ions. Cations with a larger charge and hydration radii smaller than the interlayer spacing of MXene (∼6 Å) demonstrate an order of magnitude slower permeation compared to single-charged cations. Our findings may open a door for developing efficient and highly selective separation membranes from 2D carbides.
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Cites
Phenomenological Theory of Ion Solvation. Effective Radii of Hydrated Ions
Nightingale, E. R. (1959) · The Journal of Physical Chemistry · doi:10.1021/j150579a011 · Cited by 3,505
Cited by
Two-Dimensional Ultrathin MXene Ceramic Nanosheets for Photothermal Conversion
Lin, H., Wang, X., Yu, L., Chen, Y., & Shi, J. (2017) · Nano Letters · doi:10.1021/acs.nanolett.6b04339 · Cited by 1,314
Effective ion sieving with Ti3C2Tx MXene membranes for production of drinking water from seawater
Ding, L., Li, L., Liu, Y., Wu, Y., Lu, Z., Deng, J., Wei, Y., Caro, J., & Wang, H. (2020) · Nature Sustainability · doi:10.1038/s41893-020-0474-0 · Cited by 804
Design principles of ion selective nanostructured membranes for the extraction of lithium ions
Razmjou, A., Asadnia, M., Hosseini, E., Habibnejad Korayem, A., & Chen, V. (2019) · Nature Communications · doi:10.1038/s41467-019-13648-7 · Cited by 616
Extraction of lithium from Chinese salt-lake brines by membranes: Design and practice
Xu, S., Song, J., Bi, Q., Chen, Q., Zhang, W.-M., Qian, Z., Zhang, L., Xu, S., Tang, N., & He, T. (2021) · Journal of Membrane Science · doi:10.1016/j.memsci.2021.119441 · Cited by 462
Selective Etching of Silicon from Ti3SiC2 (MAX) To Obtain 2D Titanium Carbide (MXene)
Alhabeb, M., Maleski, K., Mathis, T. S., Sarycheva, A., Hatter, C. B., Uzun, S., Levitt, A., & Gogotsi, Y. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201802232 · Cited by 452
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Metadata
- Authors
- Ren, C. E., Hatzell, K. B., Alhabeb, M., Ling, Z., Mahmoud, K. A., & Gogotsi, Y.
- Venue
- The Journal of Physical Chemistry Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-09-25
- Volume
- 6
- Issue
- 20
- Pages
- 4026-4031
- ISSN
- 1948-7185 (ISSN-L)
- OpenAlex
- W2214024197
- Cited by
- 1,030
- References
- 1
- FWCI
- 33.02
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Ren, C. E., Hatzell, K. B., Alhabeb, M., Ling, Z., Mahmoud, K. A., & Gogotsi, Y. (2015). Charge- and Size-Selective Ion Sieving Through Ti3C2Tx MXene Membranes. The Journal of Physical Chemistry Letters. https://doi.org/10.1021/acs.jpclett.5b01895
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