The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Phonon–Electron Scattering Limits Free Charge Mobility in Methylammonium Lead Iodide Perovskites
Abstract
The nature of the photoconductivity in solution-processed films of methylammonium lead iodide perovskite is investigated by determining the variation of the photoconductive response with temperature. Ultrabroadband terahertz (THz) photoconductivity spectra in the 0.3-10 THz range can be reproduced well by a simple Drude-like response at room temperature, where free charge carrier motion is characterized by an average scattering time. The scattering time determined from Drude fits in the 0.3-2THz region increases from ∼4 fs at 300 K (tetragonal phase; mobility of ∼27 cm(2) V(-1) s(-1)) to almost ∼25 fs at 77 K (orthorhombic phase, mobility of ∼150 cm(2) V(-1) s(-1)). For the tetragonal phase (temperature range 150 < T < 300 K) the scattering time shows a ∼T(-3/2) dependence, approaching the theoretical limit for pure acoustic phonon (deformation potential) scattering. Hence, electron-phonon, rather than impurity scattering, sets the upper limit on free charge transport for this perovskite.
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Stranks, S. D., Eperon, G. E., Grancini, G., Menelaou, C., Alcocer, M. J. P., Leijtens, T., Herz, L. M., Petrozza, A., & Snaith, H. J. (2013) · Science · doi:10.1126/science.1243982 · Cited by 10,413
Impact of microstructure on local carrier lifetime in perovskite solar cells
de Quilettes, D. W., Vorpahl, S. M., Stranks, S. D., Nagaoka, H., Eperon, G. E., Ziffer, M. E., Snaith, H. J., & Ginger, D. S. (2015) · Science · doi:10.1126/science.aaa5333 · Cited by 2,198
Carrier dynamics in semiconductors studied with time-resolved terahertz spectroscopy
Ulbricht, R., Hendry, E., Shan, J., Heinz, T. F., & Bonn, M. (2011) · Reviews of Modern Physics · doi:10.1103/revmodphys.83.543 · Cited by 1,293
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Cited by
Brenner, T. M., Egger, D. A., Kronik, L., Hodes, G., & Cahen, D. (2016) · Nature Reviews Materials · doi:10.1038/natrevmats.2015.7 · Cited by 1,557
Electron–phonon coupling in hybrid lead halide perovskites
Wright, A. D., Verdi, C., Milot, R. L., Eperon, G. E., Pérez-Osorio, M. A., Snaith, H. J., Giustino, F., Johnston, M. B., & Herz, L. M. (2016) · Nature Communications · doi:10.1038/ncomms11755 · Cited by 1,374
Ahmadi, M., Wu, T., & Hu, B. (2017) · Advanced Materials · doi:10.1002/adma.201605242 · Cited by 820
Causes and Solutions of Recombination in Perovskite Solar Cells
Chen, J., & Park, N. (2019) · Advanced Materials · doi:10.1002/adma.201803019 · Cited by 733
Efficient calculation of carrier scattering rates from first principles
Ganose, A. M., Park, J., Faghaninia, A., Woods-Robinson, R., Persson, K. A., & Jain, A. (2021) · Nature Communications · doi:10.1038/s41467-021-22440-5 · Cited by 688
Metadata
- Authors
- Karakus, M., Jensen, S. A., D’Angelo, F., Turchinovich, D., Bonn, M., & Cánovas, E.
- Venue
- The Journal of Physical Chemistry Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-12-04
- Volume
- 6
- Issue
- 24
- Pages
- 4991-4996
- ISSN
- 1948-7185 (ISSN-L)
- OpenAlex
- W2332088835
- Cited by
- 220
- References
- 3
- FWCI
- 14.92
- Type
- journal article
- Language
- en
- Open access
- closed
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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