The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Electron–phonon coupling in hybrid lead halide perovskites
Open accessAbstract
Phonon scattering limits charge-carrier mobilities and governs emission line broadening in hybrid metal halide perovskites. Establishing how charge carriers interact with phonons in these materials is therefore essential for the development of high-efficiency perovskite photovoltaics and low-cost lasers. Here we investigate the temperature dependence of emission line broadening in the four commonly studied formamidinium and methylammonium perovskites, HC(NH 2)2 PbI 3, HC(NH 2)2 PbBr 3, CH 3 NH 3 PbI 3 and CH 3 NH 3 PbBr 3, and discover that scattering from longitudinal optical phonons via the Fröhlich interaction is the dominant source of electron–phonon coupling near room temperature, with scattering off acoustic phonons negligible. We determine energies for the interacting longitudinal optical phonon modes to be 11.5 and 15.3 meV, and Fröhlich coupling constants of ∼40 and 60 meV for the lead iodide and bromide perovskites, respectively. Our findings correlate well with first-principles calculations based on many-body perturbation theory, which underlines the suitability of an electronic band-structure picture for describing charge carriers in hybrid perovskites.
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Stranks, S. D., Eperon, G. E., Grancini, G., Menelaou, C., Alcocer, M. J. P., Leijtens, T., Herz, L. M., Petrozza, A., & Snaith, H. J. (2013) · Science · doi:10.1126/science.1243982 · Cited by 10,413
Self-citationPrice, M. B., Butkus, J., Jellicoe, T. C., Sadhanala, A., Briane, A., Halpert, J. E., Broch, K., Hodgkiss, J. M., Friend, R. H., & Deschler, F. (2015) · Nature Communications · doi:10.1038/ncomms9420 · Cited by 704
Cited by
Leng, M., Yang, Y., Zeng, K., Chen, Z., Tan, Z., Li, S., Li, J., Xu, B., Li, D., Hautzinger, M. P., et al. (2018) · Advanced Functional Materials · doi:10.1002/adfm.201704446 · Cited by 533
Optical phonons in methylammonium lead halide perovskites and implications for charge transport
Sendner, M., Nayak, P. K., Egger, D. A., Beck, S., Müller, C., Epding, B., Kowalsky, W., Kronik, L., Snaith, H. J., Pucci, A., et al. (2016) · Materials Horizons · doi:10.1039/c6mh00275g · Cited by 403
Self-citationCrystallization of CsPbBr3 single crystals in water for X-ray detection
Peng, J., Xia, C. Q., Xu, Y., Li, R., Cui, L., Clegg, J. K., Herz, L. M., Johnston, M. B., & Lin, Q. (2021) · Nature Communications · doi:10.1038/s41467-021-21805-0 · Cited by 325
Self-citationImpact of the Organic Cation on the Optoelectronic Properties of Formamidinium Lead Triiodide
Davies, C. L., Borchert, J., Xia, C. Q., Milot, R. L., Kraus, H., Johnston, M. B., & Herz, L. M. (2018) · The Journal of Physical Chemistry Letters · doi:10.1021/acs.jpclett.8b01628 · Cited by 68
Self-citationHigh-bandwidth perovskite photonic sources on silicon
Ren, A., Wang, H., Dai, L., Xia, J., Bai, X., Butler-Caddle, E., Smith, J. A., Lai, H., Ye, J., Li, X., et al. (2023) · Nature Photonics · doi:10.1038/s41566-023-01242-9 · Cited by 49
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Metadata
- Authors
- Wright, A. D., Verdi, C., Milot, R. L., Eperon, G. E., Pérez-Osorio, M. A., Snaith, H. J., Giustino, F., Johnston, M. B., & Herz, L. M.
- Venue
- Nature Communications
- Published
- 2016-05-26
- Volume
- 7
- Issue
- 1
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2395081394
- Cited by
- 1,374
- References
- 2
- FWCI
- 54.43
- Type
- journal article
- Language
- en
- Open access
- gold
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- Wright, A. D., Verdi, C., Milot, R. L., Eperon, G. E., Pérez-Osorio, M. A., Snaith, H. J., Giustino, F., Johnston, M. B., & Herz, L. M. (2016). Electron–phonon coupling in hybrid lead halide perovskites. Nature Communications. https://doi.org/10.1038/ncomms11755
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