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Inverse Oxide/Metal Catalysts in Fundamental Studies and Practical Applications: A Perspective of Recent Developments
Open accessAbstract
Inverse oxide/metal catalysts have shown to be excellent systems for studying the role of the oxide and oxide-metal interface in catalytic reactions. These systems can have special structural and catalytic properties due to strong oxide-metal interactions difficult to attain when depositing a metal on a regular oxide support. Oxide phases that are not seen or are metastable in a bulk oxide can become stable in an oxide/metal system opening the possibility for new chemical properties. Using these systems, it has been possible to explore fundamental properties of the metal-oxide interface (composition, structure, electronic state), which determine catalytic performance in the oxidation of CO, the water-gas shift and the hydrogenation of CO2 to methanol. Recently, there has been a significant advance in the preparation of oxide/metal catalysts for technical or industrial applications. One goal is to identify methods able to control in a precise way the size of the deposited oxide particles and their structure on the metal substrate.
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Cites
Identification of Active Edge Sites for Electrochemical H 2 Evolution from MoS 2 Nanocatalysts
Jaramillo, T. F., Jørgensen, K. P., Bonde, J., Nielsen, J. H., Horch, S., & Chorkendorff, I. (2007) · Science · doi:10.1126/science.1141483 · Cited by 6,100
Cited by
Li, Y., Zhang, Y., Qian, K., & Huang, W. (2022) · ACS Catalysis · doi:10.1021/acscatal.1c04854 · Cited by 538
Metal–support interactions in metal oxide-supported atomic, cluster, and nanoparticle catalysis
Leybo, D., Etim, U. J., Monai, M., Bare, S. R., Zhong, Z., & Vogt, C. (2024) · Chemical Society Reviews · doi:10.1039/d4cs00527a · Cited by 417
Metadata
- Authors
- Rodriguez, J. A., Liu, P., Graciani, J., Senanayake, S. D., Grinter, D. C., Stacchiola, D., Hrbek, J., & Fernández-Sanz, J.
- Venue
- The Journal of Physical Chemistry Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-06-28
- Volume
- 7
- Issue
- 13
- Pages
- 2627-2639
- ISSN
- 1948-7185 (ISSN-L)
- OpenAlex
- W2470246762
- Cited by
- 168
- References
- 1
- FWCI
- 6.84
- Type
- journal article
- Language
- en
- Open access
- green
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- Rodriguez, J. A., Liu, P., Graciani, J., Senanayake, S. D., Grinter, D. C., Stacchiola, D., Hrbek, J., & Fernández-Sanz, J. (2016). Inverse Oxide/Metal Catalysts in Fundamental Studies and Practical Applications: A Perspective of Recent Developments. The Journal of Physical Chemistry Letters. https://doi.org/10.1021/acs.jpclett.6b00499
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