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The Alkaline Dissolution Rate of Calcite
Open accessAbstract
Due to the widespread presence of calcium carbonate on Earth, several geochemical systems, among which is the global CO2 cycle, are controlled to a large extent by the dissolution and precipitation of this mineral. For this reason, the dissolution of calcite has been thoroughly investigated for decades. Despite this intense activity, a consensual value of the dissolution rate of calcite has not been found yet. We show here that the inconsistency between the reported values stems mainly from the variability of the chemical and hydrodynamic conditions of measurement. The spreading of the values, when compared in identical conditions, is much less than expected and is interpreted in terms of sample surface topography. This analysis leads us to propose benchmark values of the alkaline dissolution rate of calcite compatible with all the published values, and a method to use them in various chemical and hydrodynamic contexts.
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“Because of the high diffusion rate at 200 °C and fast calcite dissolution39,40, protodolomite formation is the rate-limiting factor.”
From Acceleration of dolomitization by zinc in saline waters (2019) · cites this paper as [40]
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Acceleration of dolomitization by zinc in saline waters
Vandeginste, V., Snell, O., Hall, M. R., Steer, E., & Vandeginste, A. (2019) · Nature Communications · doi:10.1038/s41467-019-09870-y · Cited by 54
Metadata
- Authors
- Colombani, J.
- Affiliations
- Lyon 1 Université (FR)
- Corresponding author
- Colombani, Jean
- ORCID
- Colombani, Jean
- Venue
- The Journal of Physical Chemistry Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-06-13
- Volume
- 7
- Issue
- 13
- Pages
- 2376-2380
- ISSN
- 1948-7185 (ISSN-L)
- OpenAlex
- W2411167658
- Cited by
- 54
- References
- 1
- Citations by year
- 2026: 4 · 2025: 4 · 2024: 4 · 2023: 4 · 2022: 4 · 2021: 5 · 2020: 7 · 2019: 7 · 2018: 9 · 2017: 5 · 2016: 1
- FWCI
- 4.58
- Type
- journal article
- Language
- en
- Open access
- green
- hal.science
- Licence
- other-oa
- Locations
- The Journal of Physical Chemistry Letters (publishedVersion)
- PubMed (publishedVersion)
- HAL (submittedVersion, other-oa)
- Topics
- Physical Sciences › Environmental Science › Environmental Engineering › CO2 Sequestration and Geologic Interactions
- Physical Sciences › Materials Science › Biomaterials › Calcium Carbonate Crystallization and Inhibition
- Physical Sciences › Earth and Planetary Sciences › Earth-Surface Processes › Karst Systems and Hydrogeology
- Keywords
- calcite dissolution, calcium carbonate, CO2 cycle, dissolution kinetics, hydrodynamic conditions
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