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Cited by 54Adhesion, Friction, and Surface InteractionsCalcium Carbonate Crystallization and InhibitionForce Microscopy Techniques and Applications

The DOI matches its Crossref record; 149 of the 153 references it cites were found in a registry or an index.

Surface Forces Apparatus Measurements of Interactions between Rough and Reactive Calcite Surfaces

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Dziadkowiec, Joanna, Javadi, Shaghayegh, Bratvold, Jon E., Nilsen, Ola, Røyne, Anja·2018·Langmuir
DOI 10.1021/acs.langmuir.8b00797
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Abstract

nm-Range forces acting between calcite surfaces in water affect macroscopic properties of carbonate rocks and calcite-based granular materials and are significantly influenced by calcite surface recrystallization. We suggest that the repulsive mechanical effects related to nm-scale surface recrystallization of calcite in water could be partially responsible for the observed decrease of cohesion in calcitic rocks saturated with water. Using the surface forces apparatus, we simultaneously followed the calcite reactivity and measured the forces in water in two surface configurations: between two rough calcite surfaces (CC) and between rough calcite and a smooth mica surface (CM). We used nm-scale rough, polycrystalline calcite films prepared by atomic layer deposition. We measured only repulsive forces in CC in CaCO 3 -saturated water, which was related to roughness and possibly to repulsive hydration effects. Adhesive or repulsive forces were measured in CM in CaCO 3 -saturated water depending on calcite roughness, and the adhesion was likely enhanced by electrostatic effects. The pull-off adhesive force in CM became stronger with time, and this increase was correlated with a decrease of roughness at contacts, the parameter which could be estimated from the measured force–distance curves. That suggested a progressive increase of real contact areas between the surfaces, caused by gradual pressure-driven deformation of calcite surface asperities during repeated loading–unloading cycles. Reactivity of calcite was affected by mass transport across nm- to μm-thick gaps between the surfaces. Major roughening was observed only for the smoothest calcite films, where gaps between two opposing surfaces were nm-thick over μm-sized areas and led to force of crystallization that could overcome confining pressures of the order of MPa. Any substantial roughening of calcite caused a significant increase of the repulsive mechanical force contribution.

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Research works printed but not linked: 2

  1. Buzgar N., 2009, Sci. Ann. AI Cuza Univ. Iasi Sect. 2, Geol., 55, 97
  2. Oosawa F., 1971, Polyelectrolytes

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Metadata

Authors
Dziadkowiec, J., Javadi, S., Bratvold, J. E., Nilsen, O., & Røyne, A.
Affiliations
University of Oslo (NO)
Corresponding author
Dziadkowiec, Joanna
ORCID
Venue
Langmuir
Publisher
American Chemical Society (ACS)
Published
2018-05-28
Volume
34
Issue
25
Pages
7248-7263
ISSN
  • 0743-7463 (ISSN-L)
  • 1520-5827
DOI
10.1021/acs.langmuir.8b00797
OpenAlex
W2805739917
Cited by
52
References
153
Citations by year
2026: 2 · 2025: 6 · 2024: 6 · 2023: 7 · 2022: 8 · 2021: 5 · 2020: 10 · 2019: 7 · 2018: 1
FWCI
3.69
Type
journal article
Language
en
Open access
Locations
  • Langmuir (publishedVersion)
  • arXiv (Cornell University) (publishedVersion)
  • PubMed (publishedVersion)
  • NORA - Norwegian Open Research Archives (submittedVersion, other-oa)
  • arXiv (Cornell University)
Funders
  • H2020 Marie Sklodowska-Curie Actions (642976)
  • National IOR center of Norway, University of Stavanger (PR-10373)
Topics
  • Physical Sciences › Engineering › Mechanics of Materials › Adhesion, Friction, and Surface Interactions
  • Physical Sciences › Materials Science › Biomaterials › Calcium Carbonate Crystallization and Inhibition
  • Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Force Microscopy Techniques and Applications
Keywords
calcite, surface recrystallization, nanoscale surface roughness, interfacial forces, atomic layer deposition, hydration forces, electrostatic adhesion, force-distance curves, real contact area, mass transfer

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