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Cited by 318

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Quasi-BIC Resonant Enhancement of Second-Harmonic Generation in WS2 Monolayers

Bernhardt, Nils, Koshelev, Kirill, White, Simon J.U., Meng, Kelvin Wong Choon, Fröch, Johannes E., Kim, Sejeong, Tran, Toan Trong, Choi, Duk-Yong, Kivshar, Yuri, Solntsev, Alexander S.·2020·Nano Letters

Abstract

Atomically thin monolayers of transition metal dichalcogenides (TMDs) have emerged as a promising class of novel materials for optoelectronics and nonlinear optics. However, the intrinsic nonlinearity of TMD monolayers is weak, limiting their functionalities for nonlinear optical processes such as frequency conversion. Here we boost the effective nonlinear susceptibility of a TMD monolayer by integrating it with a resonant dielectric metasurface that supports pronounced optical resonances with high quality factors: bound states in the continuum (BICs). We demonstrate that a WS 2 monolayer combined with a silicon metasurface hosting BICs exhibits enhanced second-harmonic intensity by more than 3 orders of magnitude relative to a WS 2 monolayer on top of a flat silicon film of the same thickness. Our work suggests a pathway to employ high-index dielectric metasurfaces as hybrid structures for enhancement of TMD nonlinearities with applications in nonlinear microscopy, optoelectronics, and signal processing.

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Metadata

Authors
Bernhardt, N., Koshelev, K., White, S. J. U., Meng, K. W. C., Fröch, J. E., Kim, S., Tran, T. T., Choi, D.-Y., Kivshar, Y., & Solntsev, A. S.
Venue
Nano Letters
Published
2020-06-12
Volume
20
Issue
7
Pages
5309-5314
ISSN
  • 1530-6984 (ISSN-L)
  • 1530-6992
OpenAlex
W3035256848
Cited by
318
References
2
FWCI
24.42
Type
journal article
Language
en
Open access
closed

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CoChat. (2026). Citation check: Quasi-BIC Resonant Enhancement of Second-Harmonic Generation in WS2 Monolayers. https://app.cochat.ai/papers/10.1021/acs.nanolett.0c01603
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Bernhardt, N., Koshelev, K., White, S. J. U., Meng, K. W. C., Fröch, J. E., Kim, S., Tran, T. T., Choi, D.-Y., Kivshar, Y., & Solntsev, A. S. (2020). Quasi-BIC Resonant Enhancement of Second-Harmonic Generation in WS2 Monolayers. Nano Letters. https://doi.org/10.1021/acs.nanolett.0c01603

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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).

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