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Surface Plasmon Enhanced Strong Exciton–Photon Coupling in Hybrid Inorganic–Organic Perovskite Nanowires
Open accessAbstract
Manipulating strong light–matter interaction in semiconductor microcavities is crucial for developing high-performance exciton polariton devices with great potential in next-generation all-solid state quantum technologies. In this work, we report surface plasmon enhanced strong exciton–photon interaction in CH 3 NH 3 PbBr 3 perovskite nanowires. Characteristic anticrossing behaviors, indicating a Rabi splitting energy up to ∼564 meV, are observed near exciton resonance in hybrid perovskite nanowire/SiO 2 /Ag cavity at room temperature. The exciton–photon coupling strength is enhanced by ∼35% on average, which is mainly attributed to surface plasmon induced localized excitation field redistribution. Further, systematic studies on SiO 2 thickness and nanowire dimension dependence of exciton–photon interaction are presented. These results provide new avenues to achieve extremely high coupling strengths and push forward the development of electrically pumped and ultralow threshold small lasers.
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Cites
Lead halide perovskite nanowire lasers with low lasing thresholds and high quality factors
Zhu, H., Fu, Y., Meng, F., Wu, X., Gong, Z., Ding, Q., Gustafsson, M. V., Trinh, M. T., Jin, S., & Zhu, X.-Y. (2015) · Nature Materials · doi:10.1038/nmat4271 · Cited by 2,836
Superfluidity of polaritons in semiconductor microcavities
Amo, A., Lefrère, J., Pigeon, S., Adrados, C., Ciuti, C., Carusotto, I., Houdré, R., Giacobino, E., & Bramati, A. (2009) · Nature Physics · doi:10.1038/nphys1364 · Cited by 1,037
Optical phonons in methylammonium lead halide perovskites and implications for charge transport
Sendner, M., Nayak, P. K., Egger, D. A., Beck, S., Müller, C., Epding, B., Kowalsky, W., Kronik, L., Snaith, H. J., Pucci, A., et al. (2016) · Materials Horizons · doi:10.1039/c6mh00275g · Cited by 403
Optical constants of CH_3NH_3PbBr_3 perovskite thin films measured by spectroscopic ellipsometry
Alias, M. S., Dursun, I., Saidaminov, M. I., Diallo, E. M., Mishra, P., Ng, T. K., Bakr, O. M., & Ooi, B. S. (2016) · Optics Express · doi:10.1364/oe.24.016586 · Cited by 135
Cited by
Fu, Y., Zhu, H., Chen, J., Hautzinger, M. P., Zhu, X.-Y., & Jin, S. (2019) · Nature Reviews Materials · doi:10.1038/s41578-019-0080-9 · Cited by 934
Self-citationStrong light–matter interactions: a new direction within chemistry
Hertzog, M., Wang, M., Mony, J., & Börjesson, K. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00193f · Cited by 444
Halide Perovskite Semiconductor Lasers: Materials, Cavity Design, and Low Threshold
Zhang, Q., Shang, Q., Su, R., Do, T. T. H., & Xiong, Q. (2021) · Nano Letters · doi:10.1021/acs.nanolett.0c03593 · Cited by 417
Self-citationPerovskite semiconductors for room-temperature exciton-polaritonics
Su, R., Fieramosca, A., Zhang, Q., Nguyen, H. S., Deleporte, E., Chen, Z., Sanvitto, D., Liew, T. C. H., & Xiong, Q. (2021) · Nature Materials · doi:10.1038/s41563-021-01035-x · Cited by 255
Self-citationRoom temperature long-range coherent exciton polariton condensate flow in lead halide perovskites
Su, R., Wang, J., Zhao, J., Xing, J., Zhao, W., Diederichs, C., Liew, T. C. H., & Xiong, Q. (2018) · Science Advances · doi:10.1126/sciadv.aau0244 · Cited by 197
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Metadata
- Authors
- Shang, Q., Zhang, S., Liu, Z., Chen, J., Yang, P., Li, C., Li, W., Zhang, Y., Xiong, Q., Liu, X., & Zhang, Q.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-05-03
- Volume
- 18
- Issue
- 6
- Pages
- 3335-3343
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W2770126715
- Cited by
- 175
- References
- 4
- FWCI
- 11.45
- Type
- journal article
- Language
- en
- Open access
- green
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- Shang, Q., Zhang, S., Liu, Z., Chen, J., Yang, P., Li, C., Li, W., Zhang, Y., Xiong, Q., Liu, X., & Zhang, Q. (2018). Surface Plasmon Enhanced Strong Exciton–Photon Coupling in Hybrid Inorganic–Organic Perovskite Nanowires. Nano Letters. https://doi.org/10.1021/acs.nanolett.7b04847
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