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Effective Suppression of Dendritic Lithium Growth Using an Ultrathin Coating of Nitrogen and Sulfur Codoped Graphene Nanosheets on Polymer Separator for Lithium Metal Batteries
Abstract
The enhanced stability of lithium metal is vital to the development of high energy density lithium batteries due to its higher specific capacity and low redox potential. Herein, we demonstrate that nitrogen and sulfur codoped graphene (NSG) nanosheets coated on a polyethylene separator stabilized the lithium electrode in lithium metal batteries by effectively suppressing dendrite growth and maintaining a uniform ionic flux on the metal surface. The ultrathin layer of NSG nanosheets also improved the dimensional stability of the polymer separator at elevated temperatures. In addition, the enhanced interfacial interaction between the NSG-coated separator and lithium metal via electrostatic attraction released the surface tension of lithium metal and suppressed the initiation of dendrite growth on lithium metal. As a result, the electrochemical performance of a lithium metal cell composed of a LiNi0.8Co0.15Al0.05O2 positive electrode with an NSG-coated separator was remarkably improved as compared to the cell with an uncoated polyethylene separator.
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Cites
Li-O2 and Li-S batteries with high energy storage
Bruce, P. G., Freunberger, S. A., Hardwick, L. J., & Tarascon, J.-M. (2012) · Nature Materials · doi:10.1038/nmat3191 · Cited by 9,479
Cited by
Reviving the lithium metal anode for high-energy batteries
Lin, D., Liu, Y., & Cui, Y. (2017) · Nature Nanotechnology · doi:10.1038/nnano.2017.16 · Cited by 6,763
Protected Lithium‐Metal Anodes in Batteries: From Liquid to Solid
Yang, C., Fu, K., Zhang, Y., Hitz, E., & Hu, L. (2017) · Advanced Materials · doi:10.1002/adma.201701169 · Cited by 757
Zhu, B., Jin, Y., Hu, X., Zheng, Q., Zhang, S., Wang, Q., & Zhu, J. (2017) · Advanced Materials · doi:10.1002/adma.201603755 · Cited by 587
High-safety separators for lithium-ion batteries and sodium-ion batteries: advances and perspective
Zhang, L., Li, X., Yang, M., & Chen, W. (2021) · Energy Storage Materials · doi:10.1016/j.ensm.2021.06.033 · Cited by 587
Lithium dendrite growth mechanisms in polymer electrolytes and prevention strategies
Barai, P., Higa, K., & Srinivasan, V. (2017) · Physical Chemistry Chemical Physics · doi:10.1039/c7cp03304d · Cited by 339
Metadata
- Authors
- Shin, W.-K., Kannan, A. G., & Kim, D.-W.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-10-19
- Volume
- 7
- Issue
- 42
- Pages
- 23700-23707
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2275137717
- Cited by
- 238
- References
- 1
- FWCI
- 11.07
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Effective Suppression of Dendritic Lithium Growth Using an Ultrathin Coating of Nitrogen and Sulfur Codoped Graphene Nanosheets on Polymer Separator for Lithium Metal Batteries. https://app.cochat.ai/papers/10.1021/acsami.5b07730
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- Shin, W.-K., Kannan, A. G., & Kim, D.-W. (2015). Effective Suppression of Dendritic Lithium Growth Using an Ultrathin Coating of Nitrogen and Sulfur Codoped Graphene Nanosheets on Polymer Separator for Lithium Metal Batteries. ACS Applied Materials & Interfaces. https://doi.org/10.1021/acsami.5b07730
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