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Cited by 269

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Highly Stretchable and Highly Conductive PEDOT:PSS/Ionic Liquid Composite Transparent Electrodes for Solution-Processed Stretchable Electronics

Teo, Mei Ying, Kim, Nara, Kee, Seyoung, Kim, Bong Seong, Kim, Geunjin, Hong, Soonil, Jung, Suhyun, Lee, Kwanghee·2017·ACS Applied Materials & Interfaces

Abstract

Stretchable conductive materials have received great attention owing to their potential for realizing next-generation stretchable electronics. However, the simultaneous achievement of excellent mechanical stretchability and high electrical conductivity as well as cost-effective fabrication has been a significant challenge. Here, we report a highly stretchable and highly conducting polymer that was obtained by incorporating an ionic liquid. When 1-ethyl-3-methylimidazolium tetracyanoborate (EMIM TCB) was added to an aqueous conducting polymer solution of poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS), it was found that EMIM TCB acts not only as a secondary dopant but also as a plasticizer for PEDOT:PSS, resulting in a high conductivity of >1000 S cm –1 with stable performance at tensile strains up to 50% and even up to 180% in combination with the prestrained substrate technique. Consequently, by exploiting the additional benefits of high transparency and solution-processability of PEDOT:PSS, we were able to fabricate a highly stretchable, semitransparent, and wholly solution-processed alternating current electroluminescent device with unimpaired performance at 50% strain by using PEDOT:PSS/EMIM TCB composite films as both bottom and top electrodes.

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Metadata

Authors
Teo, M. Y., Kim, N., Kee, S., Kim, B. S., Kim, G., Hong, S., Jung, S., & Lee, K.
Venue
ACS Applied Materials & Interfaces
Published
2016-12-27
Volume
9
Issue
1
Pages
819-826
ISSN
  • 1944-8244 (ISSN-L)
  • 1944-8252
OpenAlex
W2567113147
Cited by
269
References
1
FWCI
14.29
Type
journal article
Language
en
Open access
closed

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CoChat. (2026). Citation check: Highly Stretchable and Highly Conductive PEDOT:PSS/Ionic Liquid Composite Transparent Electrodes for Solution-Processed Stretchable Electronics. https://app.cochat.ai/papers/10.1021/acsami.6b11988
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Teo, M. Y., Kim, N., Kee, S., Kim, B. S., Kim, G., Hong, S., Jung, S., & Lee, K. (2017). Highly Stretchable and Highly Conductive PEDOT:PSS/Ionic Liquid Composite Transparent Electrodes for Solution-Processed Stretchable Electronics. ACS Applied Materials & Interfaces. https://doi.org/10.1021/acsami.6b11988

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