The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Porous MOF with Highly Efficient Selectivity and Chemical Conversion for CO2
Abstract
A new Co(II)-based MOF, {[Co 2 (tzpa)(OH)(H 2 O) 2 ]·DMF} n ( 1 ) (H 3 tzpa = 5-(4-(tetrazol-5-yl)phenyl)isophthalic acid), was constructed by employing a tetrazolyl-carboxyl ligand H 3 tzpa. 1 possesses 1D tubular channels that are decorated by μ 3 –OH groups, uncoordinated carboxylate O atoms, and open metal centers generated by the removal of coordinated water molecules, leading to high CO 2 adsorption capacity and significantly selective capture for CO 2 over CH 4 and CO in the temperature range of 298–333 K. Moreover, 1 shows the chemical stability in acidic and basic aqueous solutions. Grand canonical Monte Carlo simulations identified multiple CO 2 -philic sites in 1 . In addition, the activated 1 as the heterogeneous Lewis and Brønsted acid bifunctional catalyst facilitates the chemical fixation of CO 2 coupling with epoxides into cyclic carbonates under ambient conditions.
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Cites
Millward, A. R., & Yaghi, O. M. (2005) · Journal of the American Chemical Society · doi:10.1021/ja0570032 · Cited by 2,876
Capture and conversion of CO2 at ambient conditions by a conjugated microporous polymer
Xie, Y., Wang, T.-T., Liu, X.-H., Zou, K., & Deng, W.-Q. (2013) · Nature Communications · doi:10.1038/ncomms2960 · Cited by 772
Cited by
Carbon capture and conversion using metal–organic frameworks and MOF-based materials
Ding, M., Flaig, R. W., Jiang, H.-L., & Yaghi, O. M. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00829a · Cited by 2,616
Kökçam-Demir, Ü., Goldman, A., Esrafili, L., Gharib, M., Morsali, A., Weingart, O., & Janiak, C. (2020) · Chemical Society Reviews · doi:10.1039/c9cs00609e · Cited by 895
Metal–organic frameworks for the chemical fixation of CO2 into cyclic carbonates
Pal, T. K., De, D., & Bharadwaj, P. K. (2020) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2019.213173 · Cited by 458
Linker functionalized metal-organic frameworks
Ali Akbar Razavi, S., & Morsali, A. (2019) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2019.213023 · Cited by 341
Recent progress in metal-organic frameworks (MOFs) for CO2 capture at different pressures
Mahajan, S., & Lahtinen, M. (2022) · Journal of Environmental Chemical Engineering · doi:10.1016/j.jece.2022.108930 · Cited by 282
Metadata
- Authors
- Wang, H.-H., Hou, L., Li, Y.-Z., Jiang, C.-Y., Wang, Y.-Y., & Zhu, Z.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-05-17
- Volume
- 9
- Issue
- 21
- Pages
- 17969-17976
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2616390082
- Cited by
- 205
- References
- 2
- FWCI
- 10.86
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wang, H.-H., Hou, L., Li, Y.-Z., Jiang, C.-Y., Wang, Y.-Y., & Zhu, Z. (2017). Porous MOF with Highly Efficient Selectivity and Chemical Conversion for CO2. ACS Applied Materials & Interfaces. https://doi.org/10.1021/acsami.7b03835
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