The DOI matches its Crossref record; 5 of the 5 references it cites were found in a registry or an index.
Healable, Reconfigurable, Reprocessable Thermoset Shape Memory Polymer with Highly Tunable Topological Rearrangement Kinetics
Abstract
The unique capability of topological rearrangement for dynamic covalent polymer networks has enabled various unusual properties (self-healing, solid-state plasticity, and reprocessability) that are not found in conventional thermosets. Achieving these properties in one network in a synergetic fashion can open up new opportunities for shape memory polymer. To accomplish such a goal, the freedom to tune topological rearrangement kinetics is critical. This is, however, challenging to achieve. In this work, two sets of dynamic bonds (urethane and hindered urea) are incorporated into a hybrid network for synthesizing shape memory poly(urea-urethane). By changing the bond ratio, networks with highly tunable topological rearrangement kinetics are obtained. Combining self-healing, solid-state plasticity, and reprocessability in one such shape memory network leads to unusual versatility in its shape-shifting performance.
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Cites
Silica-Like Malleable Materials from Permanent Organic Networks
Montarnal, D., Capelot, M., Tournilhac, F., & Leibler, L. (2011) · Science · doi:10.1126/science.1212648 · Cited by 3,625
Dynamic Covalent Polymer Networks: from Old Chemistry to Modern Day Innovations
Zou, W., Dong, J., Luo, Y., Zhao, Q., & Xie, T. (2017) · Advanced Materials · doi:10.1002/adma.201606100 · Cited by 1,014
Self-citationMechanically Activated, Catalyst-Free Polyhydroxyurethane Vitrimers
Fortman, D. J., Brutman, J. P., Cramer, C. J., Hillmyer, M. A., & Dichtel, W. R. (2015) · Journal of the American Chemical Society · doi:10.1021/jacs.5b08084 · Cited by 811
Making Insoluble Polymer Networks Malleable via Olefin Metathesis
Lu, Y.-X., Tournilhac, F., Leibler, L., & Guan, Z. (2012) · Journal of the American Chemical Society · doi:10.1021/ja303356z · Cited by 568
Shape memory polymer network with thermally distinct elasticity and plasticity
Zhao, Q., Zou, W., Luo, Y., & Xie, T. (2016) · Science Advances · doi:10.1126/sciadv.1501297 · Cited by 514
Self-citation
Cited by
Li, L., Chen, X., Jin, K., & Torkelson, J. M. (2018) · Macromolecules · doi:10.1021/acs.macromol.8b00922 · Cited by 424
Malleable and Recyclable Thermosets: The Next Generation of Plastics
Jin, Y., Lei, Z., Taynton, P., Huang, S., & Zhang, W. (2019) · Matter · doi:10.1016/j.matt.2019.09.004 · Cited by 359
Elastic vitrimers: Beyond thermoplastic and thermoset elastomers
Luo, J., Demchuk, Z., Zhao, X., Saito, T., Tian, M., Sokolov, A. P., & Cao, P.-F. (2022) · Matter · doi:10.1016/j.matt.2022.04.007 · Cited by 281
High-Performance Lignin-Containing Polyurethane Elastomers with Dynamic Covalent Polymer Networks
Liu, W., Fang, C., Wang, S., Huang, J., & Qiu, X. (2019) · Macromolecules · doi:10.1021/acs.macromol.9b01413 · Cited by 258
Li, L., Chen, X., & Torkelson, J. M. (2019) · Macromolecules · doi:10.1021/acs.macromol.9b01359 · Cited by 224
Metadata
- Authors
- Fang, Z., Zheng, N., Zhao, Q., & Xie, T.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-06-26
- Volume
- 9
- Issue
- 27
- Pages
- 22077-22082
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2660587980
- Cited by
- 222
- References
- 5
- FWCI
- 14.05
- Type
- journal article
- Language
- en
- Open access
- closed
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- Fang, Z., Zheng, N., Zhao, Q., & Xie, T. (2017). Healable, Reconfigurable, Reprocessable Thermoset Shape Memory Polymer with Highly Tunable Topological Rearrangement Kinetics. ACS Applied Materials & Interfaces. https://doi.org/10.1021/acsami.7b05713
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