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Manganese-Modified Fe3O4 Microsphere Catalyst with Effective Active Phase of Forming Light Olefins from Syngas
Abstract
A manganese-modified Fe 3 O 4 microsphere catalyst was developed, which effectively converts the syngas to light olefins (C 2 –C 4 ) with selectivity up to 60.1% in all hydrocarbon products. This nonporous catalytic material with fine dispersed manganese contributes to clarifying the different role of iron carbides by solely modifying the carburization of the catalysts and reducing the diffusion resistance of products. Combining various characterization results, including XAFS and Mössbauer spectroscopy, it is found that the electronic state of surface carbonaceous species was affected by the Mn promoter, leading to the formation of special iron carbide (θ-Fe 3 C), and the reactivity for light olefins formation was highly dependent on the content of θ-Fe 3 C.
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Sing, K. S. W. (1985) · Pure and Applied Chemistry · doi:10.1351/pac198557040603 · Cited by 24,485
Cited by
Cobalt carbide nanoprisms for direct production of lower olefins from syngas
Zhong, L., Yu, F., An, Y., Zhao, Y., Sun, Y., Li, Z., Lin, T., Lin, Y., Qi, X., Dai, Y., et al. (2016) · Nature · doi:10.1038/nature19786 · Cited by 874
Zhao, Y., Waterhouse, G. I. N., Chen, G., Xiong, X., Wu, L.-Z., Tung, C.-H., & Zhang, T. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00607e · Cited by 435
Abbas, M., Zhang, J., Mansour, T. S., & Chen, J. (2020) · International Journal of Hydrogen Energy · doi:10.1016/j.ijhydene.2020.02.044 · Cited by 32
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Metadata
- Authors
- Liu, Y., Chen, J.-F., Bao, J., & Zhang, Y.
- Venue
- ACS Catalysis
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-05-28
- Volume
- 5
- Issue
- 6
- Pages
- 3905-3909
- ISSN
- 2155-5435 (ISSN-L)
- OpenAlex
- W2509645054
- Cited by
- 236
- References
- 1
- FWCI
- 5.26
- Type
- journal article
- Language
- en
- Open access
- closed
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- Liu, Y., Chen, J.-F., Bao, J., & Zhang, Y. (2015). Manganese-Modified Fe3O4 Microsphere Catalyst with Effective Active Phase of Forming Light Olefins from Syngas. ACS Catalysis. https://doi.org/10.1021/acscatal.5b00492
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