The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Construction of Graphitic C3N4-Based Intramolecular Donor–Acceptor Conjugated Copolymers for Photocatalytic Hydrogen Evolution
Abstract
The construction of intramolecular donor–acceptor conjugated copolymers has been devised for years to enhance the mobility of charge carriers in an organic photovoltaic field; however, surprisingly, similar strategies have not been reported in polymeric photocatalytic systems for promoting the separation of charge carriers. Graphitic carbon nitride (g-C 3 N 4 ) is an emerging polymeric visible-light photocatalyst with high stability but still low photocatalytic efficiency. Here, we prepared a series of g-C 3 N 4 -based intramolecular donor–acceptor copolymers (aromatics-incorporated g-C 3 N 4 ) via nucleophilic substitution/addition reactions. The copolymer showed remarkably enhanced and stable visible-light photocatalytic hydrogen evolution performance. The intramolecular charge transfer transition is first proposed to explain the photocatalytic activity of g-C 3 N 4 -based photocatalysts under long-wavelength-light irradiation.
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Cites
Semiconductor-based Photocatalytic Hydrogen Generation
Chen, X., Shen, S., Guo, L., & Mao, S. S. (2010) · Chemical Reviews · doi:10.1021/cr1001645 · Cited by 7,876
Conjugated Polymer-Based Organic Solar Cells
Günes, S., Neugebauer, H., & Sariciftci, N. S. (2007) · Chemical Reviews · doi:10.1021/cr050149z · Cited by 6,279
Metal-free efficient photocatalyst for stable visible water splitting via a two-electron pathway
Liu, J., Liu, Y., Liu, N., Han, Y., Zhang, X., Huang, H., Lifshitz, Y., Lee, S.-T., Zhong, J., & Kang, Z. (2015) · Science · doi:10.1126/science.aaa3145 · Cited by 4,468
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Cited by
Ong, W.-J., Tan, L.-L., Ng, Y. H., Yong, S.-T., & Chai, S.-P. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00075 · Cited by 7,147
Reddy, K. R., Reddy, C. V., Nadagouda, M. N., Shetti, N. P., Jaesool, S., & Aminabhavi, T. M. (2019) · Journal of Environmental Management · doi:10.1016/j.jenvman.2019.02.075 · Cited by 429
Chen, H., Shen, K., Mao, Q., Chen, J., & Li, Y. (2018) · ACS Catalysis · doi:10.1021/acscatal.7b03270 · Cited by 341
Functional Carbon Nitride Materials in Photo‐Fenton‐Like Catalysis for Environmental Remediation
Lin, J., Tian, W., Guan, Z., Zhang, H., Duan, X., Wang, H., Sun, H., Fang, Y., Huang, Y., & Wang, S. (2022) · Advanced Functional Materials · doi:10.1002/adfm.202201743 · Cited by 303
Metadata
- Authors
- Fan, X., Zhang, L., Cheng, R., Wang, M., Li, M., Zhou, Y., & Shi, J.
- Venue
- ACS Catalysis
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-07-30
- Volume
- 5
- Issue
- 9
- Pages
- 5008-5015
- ISSN
- 2155-5435 (ISSN-L)
- OpenAlex
- W2344538577
- Cited by
- 334
- References
- 4
- FWCI
- 8.50
- Type
- journal article
- Language
- en
- Open access
- closed
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- Fan, X., Zhang, L., Cheng, R., Wang, M., Li, M., Zhou, Y., & Shi, J. (2015). Construction of Graphitic C3N4-Based Intramolecular Donor–Acceptor Conjugated Copolymers for Photocatalytic Hydrogen Evolution. ACS Catalysis. https://doi.org/10.1021/acscatal.5b01155
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