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Visible-Light Photocatalysis of Aerobic Oxidation Reactions Using Carbazolic Conjugated Microporous Polymers
Abstract
Carbazolic conjugated microporous polymer (C-CMP) is obtained via straightforward carbazole-based oxidative coupling polymerization. C-CMP exhibits high porosity and a specific surface area of 1137 m 2 g –1, and it is thermally stable to 600 °C in nitrogen. C-CMP is shown to be a highly effective heterogeneous photocatalyst for a wide range of reactions, including the oxidative coupling of primary amines, aerobic dehydrogenation of nonactive secondary amine substrates such as pharmaceutically relevant nitrogen heterocycles, and selective oxidation of sulfide using molecular oxygen and visible light. This work highlights the potential of developing photoactive N-containing CMPs as a highly stable, molecularly tunable, reusable, and metal-free visible light photocatalysts for a wide variety of organic transformations.
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Prier, C. K., Rankic, D. A., & MacMillan, D. W. C. (2013) · Chemical Reviews · doi:10.1021/cr300503r · Cited by 9,590
Cited by
Direct Z-scheme photocatalysts: Principles, synthesis, and applications
Xu, Q., Zhang, L., Yu, J., Wageh, S., Al-Ghamdi, A. A., & Jaroniec, M. (2018) · Materials Today · doi:10.1016/j.mattod.2018.04.008 · Cited by 1,635
Chen, R., Shi, J., Ma, Y., Lin, G., Lang, X., & Wang, C. (2019) · Angewandte Chemie International Edition · doi:10.1002/anie.201902543 · Cited by 697
Conjugated polymers for visible-light-driven photocatalysis
Dai, C., & Liu, B. (2020) · Energy & Environmental Science · doi:10.1039/c9ee01935a · Cited by 687
Sharma, R. K., Yadav, P., Yadav, M., Gupta, R., Rana, P., Srivastava, A., Zbořil, R., Varma, R. S., Antonietti, M., & Gawande, M. B. (2020) · Materials Horizons · doi:10.1039/c9mh00856j · Cited by 455
Porous organic polymers: a promising platform for efficient photocatalysis
Zhang, T., Xing, G., Chen, W., & Chen, L. (2020) · Materials Chemistry Frontiers · doi:10.1039/c9qm00633h · Cited by 420
Metadata
- Authors
- Su, C., Tandiana, R., Tian, B., Sengupta, A., Tang, W., Su, J., & Loh, K. P.
- Venue
- ACS Catalysis
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-05-05
- Volume
- 6
- Issue
- 6
- Pages
- 3594-3599
- ISSN
- 2155-5435 (ISSN-L)
- OpenAlex
- W2343575748
- Cited by
- 231
- References
- 1
- FWCI
- 12.22
- Type
- journal article
- Language
- en
- Open access
- closed
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