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A Titanium–Organic Framework: Engineering of the Band-Gap Energy for Photocatalytic Property Enhancement
Abstract
A visible-light-responsive metal–organic framework based on titanium hexameric cluster and high conjugation system of organic linker building block termed MOF-902 was synthesized and fully characterized. The photocatalytic properties of MOF-902 were investigated in the polymerization reaction with various monomers such as methyl methacrylate (MMA), benzyl methacrylate (BMA), and styrene (St), respectively. Gel permeation chromatography (GPC) analysis results demonstrated the high performance of MOF-902 as a catalyst, affording polymer products with high molecular weight ( M n ) and low polydispersity index (PDI). The photocatalytic efficiency of MOF-902 in the polymerization transformation obviously exceeds other catalysts such as MOF-901, UiO-66, UiO-66-NH 2, MIL-125(Ti), MIL-125-NH 2 (Ti), and commercial P25-TiO 2 .
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Cited by
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Li, X., Yang, X., Xue, H., Pang, H., & Xu, Q. (2020) · EnergyChem · doi:10.1016/j.enchem.2020.100027 · Cited by 706
Stable Metal–Organic Frameworks with Group 4 Metals: Current Status and Trends
Yuan, S., Qin, J.-S., Lollar, C. T., & Zhou, H.-C. (2018) · ACS Central Science · doi:10.1021/acscentsci.8b00073 · Cited by 561
Synthetic strategies, diverse structures and tuneable properties of polyoxo-titanium clusters
Fang, W.-H., Zhang, L., & Zhang, J. (2018) · Chemical Society Reviews · doi:10.1039/c7cs00511c · Cited by 348
Yan, Y., Li, C., Wu, Y., Gao, J., & Zhang, Q. (2020) · Journal of Materials Chemistry A · doi:10.1039/d0ta03749d · Cited by 260
Formation of CX Bonds in CO2 Chemical Fixation Catalyzed by Metal−Organic Frameworks
Hou, S., Dong, J., & Zhao, B. (2020) · Advanced Materials · doi:10.1002/adma.201806163 · Cited by 142
Metadata
- Authors
- Nguyen, H. L., Vu, T. T., Le, D., Doan, T. L. H., Nguyen, V. Q., & Phan, N. T. S.
- Venue
- ACS Catalysis
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-12-09
- Volume
- 7
- Issue
- 1
- Pages
- 338-342
- ISSN
- 2155-5435 (ISSN-L)
- OpenAlex
- W2560061537
- Cited by
- 175
- References
- 0
- FWCI
- 5.41
- Type
- journal article
- Language
- en
- Open access
- closed
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- Nguyen, H. L., Vu, T. T., Le, D., Doan, T. L. H., Nguyen, V. Q., & Phan, N. T. S. (2017). A Titanium–Organic Framework: Engineering of the Band-Gap Energy for Photocatalytic Property Enhancement. ACS Catalysis. https://doi.org/10.1021/acscatal.6b02642
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