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Highly Efficient Perovskite Solar Modules by Scalable Fabrication and Interconnection Optimization

Open access
Yang, Mengjin, Kim, Dong Hoe, Klein, Talysa R., Li, Zhen, Reese, Matthew O., Tremolet de Villers, Bertrand J., Berry, Joseph J., van Hest, Maikel F. A. M., Zhu, Kai·2018·ACS Energy Letters

Abstract

To push perovskite solar cell (PSC) technology toward practical applications, large-area perovskite solar modules with multiple subcells need to be developed by fully scalable deposition approaches. Here, we demonstrate a deposition scheme for perovskite module fabrication with spray coating of a TiO 2 electron transport layer (ETL) and blade coating of both a perovskite absorber layer and a spiro-OMeTAD-based hole transport layer (HTL). The TiO 2 ETL remaining in the interconnection between subcells significantly affects the module performance. Reducing the TiO 2 thickness changes the interconnection contact from a Schottky diode to ohmic behavior. Owing to interconnection resistance reduction, the perovskite modules with a 10 nm TiO 2 layer show enhanced performance mainly associated with an improved fill factor. Finally, we demonstrate a four-cell MA 0.7 FA 0.3 PbI 3 perovskite module with a stabilized power conversion efficiency (PCE) of 15.6% measured from an aperture area of ∼10.36 cm 2, corresponding to an active-area module PCE of 17.9% with a geometric fill factor of ∼87.3%.

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Metadata

Authors
Yang, M., Kim, D. H., Klein, T. R., Li, Z., Reese, M. O., Tremolet de Villers, B. J., Berry, J. J., van Hest, M. F. A. M., & Zhu, K.
Venue
ACS Energy Letters
Published
2018-01-09
Volume
3
Issue
2
Pages
322-328
ISSN
2380-8195 (ISSN-L)
OpenAlex
W2782049574
Cited by
192
References
1
FWCI
10.82
Type
journal article
Language
en
Open access
green

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CoChat. (2026). Citation check: Highly Efficient Perovskite Solar Modules by Scalable Fabrication and Interconnection Optimization. https://app.cochat.ai/papers/10.1021/acsenergylett.7b01221
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Yang, M., Kim, D. H., Klein, T. R., Li, Z., Reese, M. O., Tremolet de Villers, B. J., Berry, J. J., van Hest, M. F. A. M., & Zhu, K. (2018). Highly Efficient Perovskite Solar Modules by Scalable Fabrication and Interconnection Optimization. ACS Energy Letters. https://doi.org/10.1021/acsenergylett.7b01221

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