The DOI matches its Crossref record; 6 of the 6 references it cites were found in a registry or an index.
Pyridinic-N-Dominated Doped Defective Graphene as a Superior Oxygen Electrocatalyst for Ultrahigh-Energy-Density Zn–Air Batteries
Abstract
Identification of catalytic sites for oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) in carbon materials remains a great challenge. Here, we construct a pyridinic-N-dominated doped graphene with abundant vacancy defects. The optimized sample with an ultrahigh pore volume (3.43 cm 3 g –1 ) exhibits unprecedented ORR activity with a half-wave potential of 0.85 V in alkaline. For the first time, density functional theory results indicate that the quadri-pyridinic N-doped carbon site synergized with a vacancy defect is the active site, which presents the lowest overpotential of 0.28 V for ORR and 0.28 V for OER. The primary Zn–air batteries display a maximum power density of 115.2 mW cm –2 and an energy density as high as 872.3 Wh kg –1 . The rechargeable Zn–air batteries illustrate a low discharge–charge overpotential and high stability (>78 h). This work provides new insight into the correlation between the N configuration synergized with a vacancy defect in electrocatalysis.
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Cites
Atomically dispersed Ni(i) as the active site for electrochemical CO2 reduction
Yang, H. B., Hung, S.-F., Liu, S., Yuan, K., Miao, S., Zhang, L., Huang, X., Wang, H.-Y., Cai, W., Chen, R., et al. (2018) · Nature Energy · doi:10.1038/s41560-017-0078-8 · Cited by 2,239
Wu, G., Santandreu, A., Kellogg, W., Gupta, S., Ogoke, O., Zhang, H., Wang, H.-L., & Dai, L. (2016) · Nano Energy · doi:10.1016/j.nanoen.2015.12.032 · Cited by 744
Qu, K., Zheng, Y., Dai, S., & Qiao, S. Z. (2016) · Nano Energy · doi:10.1016/j.nanoen.2015.11.027 · Cited by 623
Higgins, D., Zamani, P., Yu, A., & Chen, Z. (2016) · Energy & Environmental Science · doi:10.1039/c5ee02474a · Cited by 525
Recent progress on graphene-based hybrid electrocatalysts
Xia, B., Yan, Y., Wang, X., & Lou, X. W. (. (2014) · Mater. Horiz. · doi:10.1039/c4mh00040d · Cited by 331
Hao, Y., Xu, Y., Liu, W., & Sun, X. (2018) · Materials Horizons · doi:10.1039/c7mh00706j · Cited by 203
Cited by
Liu, R., Tan, K. T., Gong, Y., Chen, Y., Li, Z., Xie, S., He, T., Lu, Z., Yang, H., & Jiang, D. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00620c · Cited by 1,083
Defect Engineering on Electrode Materials for Rechargeable Batteries
Zhang, Y., Tao, L., Xie, C., Wang, D., Zou, Y., Chen, R., Wang, Y., Jia, C., & Wang, S. (2020) · Advanced Materials · doi:10.1002/adma.201905923 · Cited by 1,019
Self-citationRecent advances in transition metal-based electrocatalysts for alkaline hydrogen evolution
Chen, Z., Duan, X., Wei, W., Wang, S., & Ni, B.-J. (2019) · Journal of Materials Chemistry A · doi:10.1039/c9ta03220g · Cited by 753
Self-citationCui, T., Wang, Y., Ye, T., Wu, J., Chen, Z., Li, J., Lei, Y., Wang, D., & Li, Y. (2022) · Angewandte Chemie International Edition · doi:10.1002/anie.202115219 · Cited by 659
Self-citationDefect engineering in earth-abundant electrocatalysts for CO2 and N2 reduction
Wang, Q., Lei, Y., Wang, D., & Li, Y. (2019) · Energy & Environmental Science · doi:10.1039/c8ee03781g · Cited by 574
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Metadata
- Authors
- Wang, Q., Ji, Y., Lei, Y., Wang, Y., Wang, Y., Li, Y., & Wang, S.
- Venue
- ACS Energy Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-04-05
- Volume
- 3
- Issue
- 5
- Pages
- 1183-1191
- ISSN
- 2380-8195 (ISSN-L)
- OpenAlex
- W2796121431
- Cited by
- 535
- References
- 6
- FWCI
- 17.31
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wang, Q., Ji, Y., Lei, Y., Wang, Y., Wang, Y., Li, Y., & Wang, S. (2018). Pyridinic-N-Dominated Doped Defective Graphene as a Superior Oxygen Electrocatalyst for Ultrahigh-Energy-Density Zn–Air Batteries. ACS Energy Letters. https://doi.org/10.1021/acsenergylett.8b00303
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