The application of graphene and its composites in oxygen reduction electrocatalysis: a perspective and review of recent progress
Abstract
This paper provides a critical review and perspective on progress realized recently towards the development of graphene-based oxygen reduction catalysts.
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Graphene-based supports doped with heteroatom species are distinct from functionalized graphene, as the foreign heteroatoms are incorporated directly into the graphitic planes.
“The graphene-based supports, doped with heteroatom species, are distinct from functionalized graphene, as the foreign heteroatoms are incorporated directly into the graphitic planes.118”
From A comprehensive review of Pt electrocatalysts for the oxygen reduction reaction: Nanostructure, activity, mechanism and carbon support in PEM fuel cells (2017) · cites this paper as [118]
The structure of the resulting SG composite could be readily controlled by fine tuning the Pt nanowire nucleation and growth reaction kinetics in addition to the Pt-support interactions.
“They revealed that the structure of the resulting composite could be readily controlled by ne tuning the Pt nanowire nucleation and growth reaction kinetics in addition to the Ptsupport interactions.118,125”
From A comprehensive review of Pt electrocatalysts for the oxygen reduction reaction: Nanostructure, activity, mechanism and carbon support in PEM fuel cells (2017) · cites this paper as [118]
Graphene has the ability to meet all criteria of ideal supports of platinum catalyst, including high surface area, electronic conductivity, electrochemical stability and the ability to distribute homogeneously uniformly sized NPs.
“Graphene has the ability to meet all criteria of ideal supports of platinum catalyst, including high surface area, electronic conductivity, electrochemical stability and the ability to distribute homogeneously uniformly sized NPs.118”
From A comprehensive review of Pt electrocatalysts for the oxygen reduction reaction: Nanostructure, activity, mechanism and carbon support in PEM fuel cells (2017) · cites this paper as [118]
Graphene and its derivatives have emerged as promising platinum electrocatalyst supports.
“Graphene and its derivatives have emerged as promising platinum electrocatalyst supports.118,120”
From A comprehensive review of Pt electrocatalysts for the oxygen reduction reaction: Nanostructure, activity, mechanism and carbon support in PEM fuel cells (2017) · cites this paper as [118]
Cites
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Graphene: Status and Prospects
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Electrocatalyst approaches and challenges for automotive fuel cells
Debe, M. K. (2012) · Nature · doi:10.1038/nature11115 · Cited by 5,885 · see citing works
High-Performance Electrocatalysts for Oxygen Reduction Derived from Polyaniline, Iron, and Cobalt
Wu, G., More, K. L., Johnston, C. M., & Zelenay, P. (2011) · Science · doi:10.1126/science.1200832 · Cited by 3,984 · see citing works
High oxygen-reduction activity and durability of nitrogen-doped graphene
Geng, D., Chen, Y., Chen, Y., Li, Y., Li, R., Sun, X., Ye, S., & Knights, S. (2011) · Energy & Environmental Science · doi:10.1039/c0ee00326c · Cited by 1,219 · see citing works
Platinum-Based Oxygen Reduction Electrocatalysts
Wu, J., & Yang, H. (2013) · Accounts of Chemical Research · doi:10.1021/ar300359w · Cited by 1,050 · see citing works
Wang, R., Higgins, D. C., Hoque, M. A., Lee, D., Hassan, F., & Chen, Z. (2013) · Scientific Reports · doi:10.1038/srep02431 · Cited by 82 · see citing works
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Sui, S., Wang, X., Zhou, X., Su, Y., Riffat, S., & Liu, C.-J. (2017) · Journal of Materials Chemistry A · doi:10.1039/c6ta08580f · Cited by 916 · see citing works
Applications of Phosphorene and Black Phosphorus in Energy Conversion and Storage Devices
Pang, J., Bachmatiuk, A., Yin, Y., Trzebicka, B., Zhao, L., Fu, L., Mendes, R. G., Gemming, T., Liu, Z., & Rummeli, M. H. (2018) · Advanced Energy Materials · doi:10.1002/aenm.201702093 · Cited by 518 · see citing works
Lao, M., Li, P., Jiang, Y., Pan, H., Dou, S. X., & Sun, W. (2022) · Nano Energy · doi:10.1016/j.nanoen.2022.107231 · Cited by 290 · see citing works
Zhu, B., Qu, C., Gao, S., Liang, Z., Zhang, H., & Zou, R. (2018) · ChemCatChem · doi:10.1002/cctc.201701691 · Cited by 35 · see citing works
- Authors
- Higgins, D., Zamani, P., Yu, A., & Chen, Z.
- Affiliations
- University of Waterloo (CA)
- Corresponding author
- Chen, Zhongwei
- Venue
- Energy & Environmental Science
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2016
- Volume
- 9
- Issue
- 2
- Pages
- 357-390
- ISSN
- 1754-5692 (ISSN-L)
- 1754-5706
- OpenAlex
- W2134459686
- Cited by
- 525
- References
- 7
- Citations by year
- 2026: 8 · 2025: 22 · 2024: 31 · 2023: 27 · 2022: 47 · 2021: 65 · 2020: 62 · 2019: 67 · 2018: 84 · 2017: 71 · 2016: 41
- FWCI
- 19.34
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Energy & Environmental Science (publishedVersion)
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Fuel Cells and Related Materials
- Physical Sciences › Materials Science › Materials Chemistry › Graphene research and applications
- Keywords
- graphene, graphene composites, oxygen reduction reaction, electrocatalysis, fuel cells, hydrogen evolution reaction, electrocatalysts
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