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Drawing a Soft Interface: An Effective Interfacial Modification Strategy for Garnet-Type Solid-State Li Batteries
Abstract
Garnet-type solid-state electrolytes (SSEs) are considered to be a good choice for solid-state batteries, yet the interfacial issues with metallic Li limit their applications. Herein, we propose an ultrasimple and effective strategy to enhance the interfacial connection between garnet SSEs and Li metal just by drawing a graphite-based soft interface with a pencil. Both experimental analysis and theoretical calculations confirm that the reaction between the graphite-based interfacial layer and metallic lithium forms a lithiated connection interface with good lithium-ionic and electronic conductivity. Compared to the reported interfacial materials, the graphite provides a soft interface with better ductility and compressibility. With improvement by this soft interface, the impedance of symmetric Li cells significantly decreases and the cell cycle is stable for over 1000 h. Moreover, a solid-state battery with Li-metal anode, ternary NCM523 cathode, and treated-garnet SSEs is fabricated and displays excellent rate capability and long cycling performance.
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Armand, M., & Tarascon, J.-M. (2008) · Nature · doi:10.1038/451652a · Cited by 19,612
A solid future for battery development
Janek, J., & Zeier, W. G. (2016) · Nature Energy · doi:10.1038/nenergy.2016.141 · Cited by 3,979
Cited by
Physicochemical Concepts of the Lithium Metal Anode in Solid-State Batteries
Krauskopf, T., Richter, F. H., Zeier, W. G., & Janek, J. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.0c00431 · Cited by 892
Recent Advances in Energy Chemistry between Solid-State Electrolyte and Safe Lithium-Metal Anodes
Cheng, X.-B., Zhao, C.-Z., Yao, Y.-X., Liu, H., & Zhang, Q. (2019) · Chem · doi:10.1016/j.chempr.2018.12.002 · Cited by 874
Artificial Interphases for Highly Stable Lithium Metal Anode
Xu, R., Cheng, X.-B., Yan, C., Zhang, X.-Q., Xiao, Y., Zhao, C.-Z., Huang, J.-Q., & Zhang, Q. (2019) · Matter · doi:10.1016/j.matt.2019.05.016 · Cited by 721
Samson, A. J., Hofstetter, K., Bag, S., & Thangadurai, V. (2019) · Energy & Environmental Science · doi:10.1039/c9ee01548e · Cited by 502
Liang, J.-Y., Zeng, X.-X., Zhang, X.-D., Zuo, T.-T., Yan, M., Yin, Y.-X., Shi, J.-L., Wu, X.-W., Guo, Y.-G., & Wan, L.-J. (2019) · Journal of the American Chemical Society · doi:10.1021/jacs.9b03517 · Cited by 404
Metadata
- Authors
- Shao, Y., Wang, H., Gong, Z., Wang, D., Zheng, B., Zhu, J., Lu, Y., Hu, Y.-S., Guo, X., Li, H., Huang, X., Yang, Y., Nan, C.-W., & Chen, L.
- Venue
- ACS Energy Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-05-01
- Volume
- 3
- Issue
- 6
- Pages
- 1212-1218
- ISSN
- 2380-8195 (ISSN-L)
- OpenAlex
- W2800619334
- Cited by
- 381
- References
- 2
- FWCI
- 18.53
- Type
- journal article
- Language
- en
- Open access
- closed
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- Shao, Y., Wang, H., Gong, Z., Wang, D., Zheng, B., Zhu, J., Lu, Y., Hu, Y.-S., Guo, X., Li, H., Huang, X., Yang, Y., Nan, C.-W., & Chen, L. (2018). Drawing a Soft Interface: An Effective Interfacial Modification Strategy for Garnet-Type Solid-State Li Batteries. ACS Energy Letters. https://doi.org/10.1021/acsenergylett.8b00453
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