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Core@Shell CsPbBr3@Zeolitic Imidazolate Framework Nanocomposite for Efficient Photocatalytic CO2 Reduction
Abstract
The proper energy band structure and excellent visible-light responses enable halide perovskites as potential photocatalysts for CO 2 reduction, but the conversion efficiency is still low due to the serious radiative recombination, low CO 2 capturing ability, and poor stability. Here we illustrate the design and synthesis of a halide perovskite@metal–organic framework (MOF) composite photocatalyst with enhanced CO 2 reduction activity. A facile in situ synthetic procedure is employed to directly grow a zinc/cobalt-based zeolitic imidazolate framework (ZIF) coating on the surface of CsPbBr 3 quantum dots. The CsPbBr 3 @ZIF composite shows largely improved moisture stability, CO 2 capturing ability, and charge separation efficiency. Moreover, the catalytic active Co centers in ZIF-67 can further accelerate the charge separation process and activate the adsorbed CO 2 molecules, which leads to enhanced catalytic activity for gaseous CO 2 reduction. This work would provide new insight for designing excellent perovskite/MOF-based catalysts.
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Xu, H.-Q., Hu, J., Wang, D., Li, Z., Zhang, Q., Luo, Y., Yu, S.-H., & Jiang, H.-L. (2015) · Journal of the American Chemical Society · doi:10.1021/jacs.5b08773 · Cited by 1,166
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Zhang, Y., Xia, B., Ran, J., Davey, K., & Qiao, S. Z. (2020) · Advanced Energy Materials · doi:10.1002/aenm.201903879 · Cited by 423
Jiang, Y., Liao, J.-F., Chen, H.-Y., Zhang, H.-H., Li, J.-Y., Wang, X.-D., & Kuang, D.-B. (2020) · Chem · doi:10.1016/j.chempr.2020.01.005 · Cited by 404
Self-citationZ‐Scheme 2D/2D Heterojunction of CsPbBr3/Bi2WO6 for Improved Photocatalytic CO2 Reduction
Jiang, Y., Chen, H., Li, J., Liao, J., Zhang, H., Wang, X., & Kuang, D. (2020) · Advanced Functional Materials · doi:10.1002/adfm.202004293 · Cited by 375
Self-citationReddy, C. V., Reddy, K. R., Harish, V. V. N., Shim, J., Shankar, M. V., Shetti, N. P., & Aminabhavi, T. M. (2020) · International Journal of Hydrogen Energy · doi:10.1016/j.ijhydene.2019.02.144 · Cited by 320
Metadata
- Authors
- Kong, Z.-C., Liao, J.-F., Dong, Y.-J., Xu, Y.-F., Chen, H.-Y., Kuang, D.-B., & Su, C.-Y.
- Venue
- ACS Energy Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-10-04
- Volume
- 3
- Issue
- 11
- Pages
- 2656-2662
- ISSN
- 2380-8195 (ISSN-L)
- OpenAlex
- W2895042724
- Cited by
- 564
- References
- 1
- FWCI
- 12.84
- Type
- journal article
- Language
- en
- Open access
- closed
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- Kong, Z.-C., Liao, J.-F., Dong, Y.-J., Xu, Y.-F., Chen, H.-Y., Kuang, D.-B., & Su, C.-Y. (2018). Core@Shell CsPbBr3@Zeolitic Imidazolate Framework Nanocomposite for Efficient Photocatalytic CO2 Reduction. ACS Energy Letters. https://doi.org/10.1021/acsenergylett.8b01658
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