Cited by 135Electrocatalysts for Energy Conversion2D Materials and ApplicationsGraphene research and applications

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MoS 2 Moiré Superlattice for Hydrogen Evolution Reaction

Jiang, Zhenzhen, Zhou, Wenda, Hong, Aijun, Guo, Manman, Luo, Xingfang, Yuan, Cailei·2019·ACS Energy Letters

DOI 10.1021/acsenergylett.9b02023

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Abstract

A MoS 2 moiré superlattice with a twisted angle of θ ≈ 7.3° via a facile method instead of a conventional mechanical stacking method is successfully fabricated. With reduced interlayer potential barriers demonstrated by first-principles calculations and ultralow frequency Raman spectra, electrons can transfer easily from a conductive substrate to active sites in this MoS 2 superlattice, thus leading to good hydrogen evolution reaction (HER) activities. By using an electrochemical microcell technique, improved catalytic performance in the MoS 2 moiré superlattice is validated, with a current density of −10 mA/cm 2 at an overpotential of −153 mV and a Tafel slope of 73 mV/dec. A strategy to boost the electrocatalytic performance by reducing the interlayer potential barriers is successfully achieved by employing a MoS 2 moiré superlattice. The work paves a new pathway to break the bottleneck for further improvement of HER performance and also opens interesting possibilities for implementing moiré superlattices in catalysis, energy storage, and 2D functional devices.

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Authors: Jiang, Z., Zhou, W., Hong, A., Guo, M., Luo, X., & Yuan, C.
Affiliations: Jiangxi Normal University (CN)
Corresponding author: Yuan, Cailei
ORCID: Jiang, Zhenzhen
Zhou, Wenda
Hong, Aijun
Guo, Manman
Luo, Xingfang
Yuan, Cailei
Venue: ACS Energy Letters
Publisher: American Chemical Society (ACS)
Published: 2019-10-30
Volume: 4
Issue: 12
Pages: 2830-2835
ISSN: 2380-8195 (ISSN-L)
DOI: 10.1021/acsenergylett.9b02023
OpenAlex: W2982461889
Cited by: 135
References: 45
Citations by year: 2026: 10 · 2025: 14 · 2024: 18 · 2023: 23 · 2022: 30 · 2021: 30 · 2020: 10
FWCI: 3.73
Type: journal article
Language: en
Open access: closed
Licence: doi.org/10.15223/policy-029 (stm-asf)
doi.org/10.15223/policy-037 (stm-asf)
doi.org/10.15223/policy-045 (stm-asf)
Locations: ACS Energy Letters (publishedVersion)
Funders: National Natural Science Foundation of China (51561012, 51661012, 51761017, 51871115)
Government of Jiangxi Province (20171BCB23033)
Natural Science Foundation of Jiangxi Province (20181BAB206001)
Topics: Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
Physical Sciences › Materials Science › Materials Chemistry › 2D Materials and Applications
Physical Sciences › Materials Science › Materials Chemistry › Graphene research and applications
Keywords: MoS2, moiré superlattices, hydrogen evolution reaction, electrocatalysis, twisted bilayers, two-dimensional materials, electrochemical microcell, Tafel slope, overpotential

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MoS 2 Moiré Superlattice for Hydrogen Evolution Reaction

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