Deformable Catalytic Material Derived from Mechanical Flexibility for Hydrogen Evolution Reaction
Open accessAbstract
Deformable catalytic material with excellent flexible structure is a new type of catalyst that has been applied in various chemical reactions, especially electrocatalytic hydrogen evolution reaction (HER). In recent years, deformable catalysts for HER have made great progress and would become a research hotspot. The catalytic activities of deformable catalysts could be adjustable by the strain engineering and surface reconfiguration. The surface curvature of flexible catalytic materials is closely related to the electrocatalytic HER properties. Here, firstly, we systematically summarized self-adaptive catalytic performance of deformable catalysts and various micro–nanostructures evolution in catalytic HER process. Secondly, a series of strategies to design highly active catalysts based on the mechanical flexibility of low-dimensional nanomaterials were summarized. Last but not least, we presented the challenges and prospects of the study of flexible and deformable micro–nanostructures of electrocatalysts, which would further deepen the understanding of catalytic mechanisms of deformable HER catalyst.
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Nanostructures with high aspect ratios or weak substrate adhesion are prone to structural collapse, detachment, or morphological degradation during long-term gas evolution or under mechanical damage.
“Secondly, nanostructures with high aspect ratios or weak substrate adhesion are prone to structural collapse, detachment, or morphological degradation during long-term gas evolution or under mechanical damage [175].”
From Advances in Surface/Interface Engineering of Under-Water Superaerophobic Electrodes for Hydrogen Evolution Reaction by Manipulating of Bubbles (2026) · cites this paper as [175]
The Introduction (page unavailable) says that fluid flow and hydrogen bubbles can deform low-dimensional catalysts and that bubble forces can break rigid materials, degrading HER performance. The Bend-restoration Nanotubes section (page unavailable) also links bubble forces to poor stability. Neither passage identifies high aspect ratio or weak substrate adhesion as risk factors, or establishes substrate detachment during long-term gas evolution. (LLM, conf=0.84)
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Flagged first, then by citations
Cited by
Sorted by citations
He, A., Chen, F., He, J., Zhang, X., Xie, S., Yao, N., Guo, Z., & Xu, W. (2026) · Nano-Micro Letters · doi:10.1007/s40820-026-02198-5 · Cited by 5 · see citing works
Zhu, Z., Qiu, J., Xie, L., & Wang, L. (2025) · Advanced Sustainable Systems · doi:10.1002/adsu.202500159 · Cited by 3 · see citing works
Self-citation
- Authors
- Wang, F., Xie, L., Sun, N., Zhi, T., Zhang, M., Liu, Y., Luo, Z., Yi, L., Zhao, Q., & Wang, L.
- Affiliations
- Nanjing University of Posts and Telecommunications (CN)
- Xiangtan University (CN)
- Corresponding author
- Zhi, Ting
- Zhao, Qiang
- Wang, Longlu
- Venue
- Nano-Micro Letters
- Published
- 2023-11-24
- Volume
- 16
- Issue
- 1
- Pages
- 32-32
- ISSN
- 2150-5551 (ISSN-L)
- 2311-6706
- PMC
- PMC10673806
- OpenAlex
- W4388971938
- Cited by
- 36
- References
- 130
- Citations by year
- 2026: 11 · 2025: 14 · 2024: 9 · 2023: 1 · 2022: 1
- FWCI
- 0.54
- Type
- journal article
- Language
- en
- Open access
- gold
- doi.org
- Locations
- Nano-Micro Letters (publishedVersion, cc-by)
- PubMed Central (publishedVersion, cc-by)
- PubMed (publishedVersion)
- DOAJ (DOAJ: Directory of Open Access Journals) (submittedVersion, cc-by-sa)
- Funders
- Shanghai Jiao Tong University
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › CO2 Reduction Techniques and Catalysts
- Physical Sciences › Materials Science › Materials Chemistry › Hydrogen Storage and Materials
- Keywords
- electrocatalytic hydrogen evolution, mechanical flexibility, strain engineering, surface curvature, low-dimensional nanostructures, micro/nanostructures, catalyst design strategies
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