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Oxygen-Bridged Stabilization of Single Atomic W on Rh Metallenes for Robust and Efficient pH-Universal Hydrogen Evolution
Abstract
Highly efficient and durable electrocatalysts are of the utmost importance for the sustainable generation of clean hydrogen by water electrolysis. Here, we present a report of an atomically thin rhodium metallene incorporated with oxygen-bridged single atomic tungsten (Rh-O-W) as a high-performance electrocatalyst for pH-universal hydrogen evolution reaction. The Rh-O-W metallene delivers ascendant electrocatalytic HER performance, characterized by exceptionally low overpotentials, ultrahigh mass activities, excellent turnover frequencies, and robust stability with negligible deactivation, in pH-universal electrolytes, outperforming that of benchmark Pt/C, Rh/C and numerous other reported precious-metal HER catalysts. Interestingly, the promoting feature of -O-W single atomic sites is understood via operando X-ray absorption spectroscopy characterization and theoretical calculations. On account of electron transfer and equilibration processes take place between the binary components of Rh-O-W metallenes, fine-tuning of the density of states and electron localization at Rh active sites is attained, hence promoting HER via a near-optimal hydrogen adsorption.
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The upshift of the Rh d-band center enhances the adsorption of HER intermediates.
“enhancing the adsorption of HER intermediates [52].”
From Rational synthesis of Au3Cu@Rhx core–shell aerogel electrocatalysts for efficient hydrogen evolution reaction (2026) · cites this paper as [52]
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Metadata
- Authors
- Prabhu, P., Do, V.-H., Peng, C. K., Hu, H., Chen, S.-Y., Choi, J.-H., Lin, Y.-G., & Lee, J.-M.
- Affiliations
- Nanyang Technological University (SG)
- National Yang Ming Chiao Tung University (TW)
- Soochow University (CN)
- National Synchrotron Radiation Research Center (TW)
- Corresponding author
- Choi, Jin-Ho
- Lin, Yan-Gu
- Lee, Jong-Min
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2023-05-17
- Volume
- 17
- Issue
- 11
- Pages
- 10733-10747
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W4376868300
- Cited by
- 117
- References
- 11
- Citations by year
- 2026: 19 · 2025: 39 · 2024: 51 · 2023: 8
- FWCI
- 5.60
- Type
- journal article
- Language
- en
- Open access
- closed
- Licence
- Locations
- ACS Nano (publishedVersion)
- PubMed (publishedVersion)
- DR-NTU (Nanyang Technological University) (submittedVersion)
- Funders
- Ministry of Education - Singapore (RG105/19)
- National Natural Science Foundation of China (11874044)
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › CO2 Reduction Techniques and Catalysts
- Physical Sciences › Materials Science › Materials Chemistry › Catalytic Processes in Materials Science
- Keywords
- hydrogen evolution reaction, pH-universal electrocatalysis, water electrolysis, hydrogen adsorption, catalyst stability, mass activity
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