The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Merging Single-Atom-Dispersed Silver and Carbon Nitride to a Joint Electronic System via Copolymerization with Silver Tricyanomethanide
Open accessAbstract
Herein, we present an approach to create a hybrid between single-atom-dispersed silver and a carbon nitride polymer. Silver tricyanomethanide (AgTCM) is used as a reactive comonomer during templated carbon nitride synthesis to introduce both negative charges and silver atoms/ions to the system. The successful introduction of the extra electron density under the formation of a delocalized joint electronic system is proven by photoluminescence measurements, X-ray photoelectron spectroscopy investigations, and measurements of surface ζ-potential. At the same time, the principal structure of the carbon nitride network is not disturbed, as shown by solid-state nuclear magnetic resonance spectroscopy and electrochemical impedance spectroscopy analysis. The synthesis also results in an improvement of the visible light absorption and the development of higher surface area in the final products. The atom-dispersed AgTCM-doped carbon nitride shows an enhanced performance in the selective hydrogenation of alkynes in comparison with the performance of other conventional Ag-based materials prepared by spray deposition and impregnation-reduction methods, here exemplified with 1-hexyne.
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Cites
Hydrogen evolution by a metal-free electrocatalyst
Zheng, Y., Jiao, Y., Zhu, Y., Li, L. H., Han, Y., Chen, Y., Du, A., Jaroniec, M., & Qiao, S. Z. (2014) · Nature Communications · doi:10.1038/ncomms4783 · Cited by 2,236
Cited by
Heterogeneous Single-Atom Photocatalysts: Fundamentals and Applications
Gao, C., Low, J., Long, R., Kong, T., Zhu, J., & Xiong, Y. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00840 · Cited by 1,050
An, S., Zhang, G., Wang, T., Zhang, W., Li, K., Song, C., Miller, J. T., Miao, S., Wang, J., & Guo, X. (2018) · ACS Nano · doi:10.1021/acsnano.8b04693 · Cited by 601
Xiao, X., Gao, Y., Zhang, L., Zhang, J., Zhang, Q., Li, Q., Bao, H., Zhou, J., Miao, S., Chen, N., et al. (2020) · Advanced Materials · doi:10.1002/adma.202003082 · Cited by 528
Chen, Z., Savateev, A., Pronkin, S., Papaefthimiou, V., Wolff, C., Willinger, M. G., Willinger, E., Neher, D., Antonietti, M., & Dontsova, D. (2017) · Advanced Materials · doi:10.1002/adma.201700555 · Cited by 363
Self-citationZeng, Y., Liu, X., Liu, C., Wang, L., Xia, Y., Zhang, S., Luo, S., & Pei, Y. (2018) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2017.10.042 · Cited by 336
Metadata
- Authors
- Chen, Z., Pronkin, S., Fellinger, T.-P., Kailasam, K., Vilé, G., Albani, D., Krumeich, F., Leary, R., Barnard, J., Thomas, J. M., Pérez-Ramírez, J., Antonietti, M., & Dontsova, D.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-02-15
- Volume
- 10
- Issue
- 3
- Pages
- 3166-3175
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W2255007534
- Cited by
- 257
- References
- 1
- FWCI
- 13.22
- Type
- journal article
- Language
- en
- Open access
- green
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- CoChat. (2026). Citation check: Merging Single-Atom-Dispersed Silver and Carbon Nitride to a Joint Electronic System via Copolymerization with Silver Tricyanomethanide. https://app.cochat.ai/papers/10.1021/acsnano.5b04210
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- Chen, Z., Pronkin, S., Fellinger, T.-P., Kailasam, K., Vilé, G., Albani, D., Krumeich, F., Leary, R., Barnard, J., Thomas, J. M., Pérez-Ramírez, J., Antonietti, M., & Dontsova, D. (2016). Merging Single-Atom-Dispersed Silver and Carbon Nitride to a Joint Electronic System via Copolymerization with Silver Tricyanomethanide. ACS Nano. https://doi.org/10.1021/acsnano.5b04210
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