The DOI matches its Crossref record; 36 of the 36 references it cites were found in a registry or an index.
Merging Single-Atom-Dispersed Silver and Carbon Nitride to a Joint Electronic System via Copolymerization with Silver Tricyanomethanide
Open accessAbstract
Herein, we present an approach to create a hybrid between single-atom-dispersed silver and a carbon nitride polymer. Silver tricyanomethanide (AgTCM) is used as a reactive comonomer during templated carbon nitride synthesis to introduce both negative charges and silver atoms/ions to the system. The successful introduction of the extra electron density under the formation of a delocalized joint electronic system is proven by photoluminescence measurements, X-ray photoelectron spectroscopy investigations, and measurements of surface ζ-potential. At the same time, the principal structure of the carbon nitride network is not disturbed, as shown by solid-state nuclear magnetic resonance spectroscopy and electrochemical impedance spectroscopy analysis. The synthesis also results in an improvement of the visible light absorption and the development of higher surface area in the final products. The atom-dispersed AgTCM-doped carbon nitride shows an enhanced performance in the selective hydrogenation of alkynes in comparison with the performance of other conventional Ag-based materials prepared by spray deposition and impregnation-reduction methods, here exemplified with 1-hexyne.
Overview
The claims and statistics of this paper haven’t been checked yet.
Run the check — free, no account needed. It reads the open-access text and checks the sources it cites.
Integrity signals
Registry
Cites
Statistics
Verification
Claims the paper makes
The claims and statistics of this paper haven’t been checked yet.
Run the check — free, no account needed. It reads the open-access text and checks the sources it cites.
Self-check
Percentages, sums and reported differences re-computed from the paper’s own numbers.
The self-check needs the paper’s full text.
Citations
Cites
A metal-free polymeric photocatalyst for hydrogen production from water under visible light
Wang, X., Maeda, K., Thomas, A., Takanabe, K., Xin, G., Carlsson, J. M., Domen, K., & Antonietti, M. (2009) · Nature Materials · doi:10.1038/nmat2317 · Cited by 12,532
Self-citationHigh-Resolution X-Ray Photoemission Spectrum of the Valence Bands of Gold
Shirley, D. A. (1972) · Physical Review B · doi:10.1103/physrevb.5.4709 · Cited by 6,231
Thomas, A., Fischer, A., Goettmann, F., Antonietti, M., Müller, J.-O., Schlögl, R., & Carlsson, J. M. (2008) · Journal of Materials Chemistry · doi:10.1039/b800274f · Cited by 3,419
Self-citationHydrogen evolution by a metal-free electrocatalyst
Zheng, Y., Jiao, Y., Zhu, Y., Li, L. H., Han, Y., Chen, Y., Du, A., Jaroniec, M., & Qiao, S. Z. (2014) · Nature Communications · doi:10.1038/ncomms4783 · Cited by 2,236
Wagner, C. D., Davis, L. E., Zeller, M. V., Taylor, J. A., Raymond, R. H., & Gale, L. H. (1981) · Surface and Interface Analysis · doi:10.1002/sia.740030506 · Cited by 2,075
Wang, X., Maeda, K., Chen, X., Takanabe, K., Domen, K., Hou, Y., Fu, X., & Antonietti, M. (2009) · Journal of the American Chemical Society · doi:10.1021/ja809307s · Cited by 1,809
Self-citationMetal‐Containing Carbon Nitride Compounds: A New Functional Organic–Metal Hybrid Material
Wang, X., Chen, X., Thomas, A., Fu, X., & Antonietti, M. (2009) · Advanced Materials · doi:10.1002/adma.200802627 · Cited by 1,333
Self-citationFree-energy density functional for hard spheres
Tarazona, P. (1985) · Physical Review A · doi:10.1103/physreva.31.2672 · Cited by 1,065
A Stable Single‐Site Palladium Catalyst for Hydrogenations
Vilé, G., Albani, D., Nachtegaal, M., Chen, Z., Dontsova, D., Antonietti, M., López, N., & Pérez‐Ramírez, J. (2015) · Angewandte Chemie International Edition · doi:10.1002/anie.201505073 · Cited by 973
Self-citationImproving Carbon Nitride Photocatalysis by Supramolecular Preorganization of Monomers
Shalom, M., Inal, S., Fettkenhauer, C., Neher, D., & Antonietti, M. (2013) · Journal of the American Chemical Society · doi:10.1021/ja402521s · Cited by 889
Self-citationMaeda, K., Wang, X., Nishihara, Y., Lu, D., Antonietti, M., & Domen, K. (2009) · The Journal of Physical Chemistry C · doi:10.1021/jp809119m · Cited by 825
Self-citationWang, Y., Yao, J., Li, H., Su, D., & Antonietti, M. (2011) · Journal of the American Chemical Society · doi:10.1021/ja109856y · Cited by 763
Self-citationGe, L., Han, C., Liu, J., & Li, Y. (2011) · Applied Catalysis A: General · doi:10.1016/j.apcata.2011.10.006 · Cited by 669
Phase equilibria of fluid interfaces and confined fluids: Non-local versus local density functionals
Tarazona, P., Marconi, U. M. B., & Evans, R. (1987) · Molecular Physics · doi:10.1080/00268978700100381 · Cited by 640
Kumar, S., Surendar, T., Baruah, A., & Shanker, V. (2013) · Journal of Materials Chemistry A · doi:10.1039/c3ta00186e · Cited by 624
Encyclopedia of Electrochemistry
(2010) · Wiley eBooks · doi:10.1002/9783527610426 · Cited by 621
High Performance Fe- and N- Doped Carbon Catalyst with Graphene Structure for Oxygen Reduction
Peng, H., Mo, Z., Liao, S., Liang, H., Yang, L., Luo, F., Song, H., Zhong, Y., & Zhang, B. (2013) · Scientific Reports · doi:10.1038/srep01765 · Cited by 601
Visible Light-Driven Pure Water Splitting by a Nature-Inspired Organic Semiconductor-Based System
Martin, D. J., Reardon, P. J. T., Moniz, S. J. A., & Tang, J. (2014) · Journal of the American Chemical Society · doi:10.1021/ja506386e · Cited by 556
Enhancement of visible photocatalytic activity via Ag@C3N4 core–shell plasmonic composite
Bai, X., Zong, R., Li, C., Liu, D., Liu, Y., & Zhu, Y. (2014) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2013.08.007 · Cited by 512
Ein stabiler “Single‐site”‐Palladiumkatalysator für Hydrierungen
Vilé, G., Albani, D., Nachtegaal, M., Chen, Z., Dontsova, D., Antonietti, M., López, N., & Pérez‐Ramírez, J. (2015) · Angewandte Chemie · doi:10.1002/ange.201505073 · Cited by 506
Self-citationKatsumata, H., Sakai, T., Suzuki, T., & Kaneco, S. (2014) · Industrial & Engineering Chemistry Research · doi:10.1021/ie5012036 · Cited by 402
Bu, Y., Chen, Z., & Li, W. (2014) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2013.07.066 · Cited by 286
Self-citationJiang, D., Chen, L., Xie, J., & Chen, M. (2014) · Dalton Trans. · doi:10.1039/c3dt53526f · Cited by 224
Yang, X., Tang, H., Xu, J., Antonietti, M., & Shalom, M. (2015) · ChemSusChem · doi:10.1002/cssc.201403168 · Cited by 204
Self-citationVilé, G., Almora‐Barrios, N., Mitchell, S., López, N., & Pérez‐Ramírez, J. (2014) · Chemistry – A European Journal · doi:10.1002/chem.201304795 · Cited by 179
Self-citationJiang, D., Zhu, J., Chen, M., & Xie, J. (2013) · Journal of Colloid and Interface Science · doi:10.1016/j.jcis.2013.11.042 · Cited by 152
Highly selective Pd@mpg-C3N4 catalyst for phenol hydrogenation in aqueous phase
Li, Y., Xu, X., Zhang, P., et al. (2013) · RSC Advances · doi:10.1039/c3ra41397g · Cited by 138
Xu, Y., & Zhang, W. (2013) · ChemCatChem · doi:10.1002/cctc.201300144 · Cited by 137
Deng, D., Yang, Y., Gong, Y., Li, Y., Xu, X., & Wang, Y. (2013) · Green Chemistry · doi:10.1039/c3gc40779a · Cited by 134
Vilé, G., Baudouin, D., Remediakis, I. N., Copéret, C., López, N., & Pérez‐Ramírez, J. (2013) · ChemCatChem · doi:10.1002/cctc.201300569 · Cited by 107
Self-citationQuantification of photocatalytic hydrogen evolution
Schwarze, M., Stellmach, D., Schröder, M., Kailasam, K., Reske, R., Thomas, A., & Schomäcker, R. (2013) · Physical Chemistry Chemical Physics · doi:10.1039/c3cp50168j · Cited by 84
Self-citationCao, J., Zhao, Y., Lin, H., Xu, B., & Chen, S. (2013) · Materials Research Bulletin · doi:10.1016/j.materresbull.2013.05.120 · Cited by 80
Jiang, D., Zhang, Y., Chu, H., Liu, J., Wan, J., & Chen, M. (2014) · RSC Advances · doi:10.1039/c4ra00601a · Cited by 78
Vilé, G., Wrabetz, S., Floryan, L., et al. (2014) · ChemCatChem · doi:10.1002/cctc.201402124 · Cited by 60
Self-citationVilé, G., & Pérez‐Ramírez, J. (2014) · Nanoscale · doi:10.1039/c4nr02777a · Cited by 42
Self-citationEnhancement of the Photocatalytic Activity of Carbon Nitrides by Complex Templating
Chen, Z., Antonietti, M., & Dontsova, D. (2015) · Chemistry - A European Journal · doi:10.1002/chem.201500579 · Cited by 28
Self-citation
Cited by
Heterogeneous Single-Atom Photocatalysts: Fundamentals and Applications
Gao, C., Low, J., Long, R., Kong, T., Zhu, J., & Xiong, Y. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00840 · Cited by 1,050
An, S., Zhang, G., Wang, T., Zhang, W., Li, K., Song, C., Miller, J. T., Miao, S., Wang, J., & Guo, X. (2018) · ACS Nano · doi:10.1021/acsnano.8b04693 · Cited by 601
Xiao, X., Gao, Y., Zhang, L., Zhang, J., Zhang, Q., Li, Q., Bao, H., Zhou, J., Miao, S., Chen, N., et al. (2020) · Advanced Materials · doi:10.1002/adma.202003082 · Cited by 528
Cao, S., Li, H., Tong, T., Chen, H., Yu, A., Yu, J., & Chen, H. M. (2018) · Advanced Functional Materials · doi:10.1002/adfm.201802169 · Cited by 438
Silver Single Atom in Carbon Nitride Catalyst for Highly Efficient Photocatalytic Hydrogen Evolution
Jiang, X., Zhang, L., Liu, H., Wu, D., Wu, F., Tian, L., Liu, L., Zou, J., Luo, S., & Chen, B. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.202011495 · Cited by 432
Metadata
- Authors
- Chen, Z., Pronkin, S., Fellinger, T.-P., Kailasam, K., Vilé, G., Albani, D., Krumeich, F., Leary, R., Barnard, J., Thomas, J. M., Pérez-Ramírez, J., Antonietti, M., & Dontsova, D.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-02-15
- Volume
- 10
- Issue
- 3
- Pages
- 3166-3175
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W2255007534
- Cited by
- 257
- References
- 36
- FWCI
- 13.22
- Type
- journal article
- Language
- en
- Open access
- green
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
What counts as a claim ›How we measure confidence ›How we check this ›
Are you an author, or do you see a problem with this page? Request a review
Data sources
Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
