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Ligand-Mediated Synthesis of Shape-Controlled Cesium Lead Halide Perovskite Nanocrystals via Reprecipitation Process at Room Temperature
Abstract
Colloidal nanocrystals of fully inorganic cesium lead halide (CsPbX3, X = Cl, Br, I, or combinations thereof) perovskites have attracted much attention for photonic and optoelectronic applications. Herein, we demonstrate a facile room-temperature (e.g., 25 °C), ligand-mediated reprecipitation strategy for systematically manipulating the shape of CsPbX3 colloidal nanocrystals, such as spherical quantum dots, nanocubes, nanorods, and nanoplatelets. The colloidal spherical quantum dots of CsPbX3 were synthesized with photoluminescence (PL) quantum yield values up to >80%, and the corresponding PL emission peaks covering the visible range from 380 to 693 nm. Besides spherical quantum dots, the shape of CsPbX3 nanocrystals could be engineered into nanocubes, one-dimensional nanorods, and two-dimensional few-unit-cell-thick nanoplatelets with well-defined morphology by choosing different organic acid and amine ligands via the reprecipitation process. The shape-dependent PL decay lifetimes have been determined to be several to tens to hundreds of nanoseconds. Our method provides a facile and versatile route to rationally control the shape of the CsPbX3 perovskites nanocrystals, which will create opportunities for applications such as displays, lasing, light-emitting diodes, solar concentrators, and photon detection.
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Akkerman, Q. A., D’Innocenzo, V., Accornero, S., Scarpellini, A., Petrozza, A., Prato, M., & Manna, L. (2015) · Journal of the American Chemical Society · doi:10.1021/jacs.5b05602 · Cited by 2,197
Cited by
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Kang, J., & Wang, L.-W. (2017) · The Journal of Physical Chemistry Letters · doi:10.1021/acs.jpclett.6b02800 · Cited by 1,305
Doping Lanthanide into Perovskite Nanocrystals: Highly Improved and Expanded Optical Properties
Pan, G., Bai, X., Yang, D., Chen, X., Jing, P., Qu, S., Zhang, L., Zhou, D., Zhu, J., Xu, W., et al. (2017) · Nano Letters · doi:10.1021/acs.nanolett.7b04575 · Cited by 935
Efficient and Stable White LEDs with Silica‐Coated Inorganic Perovskite Quantum Dots
Sun, C., Zhang, Y., Ruan, C., Yin, C., Wang, X., Wang, Y., & Yu, W. W. (2016) · Advanced Materials · doi:10.1002/adma.201603081 · Cited by 934
van der Stam, W., Geuchies, J. J., Altantzis, T., van den Bos, K. H. W., Meeldijk, J. D., Van Aert, S., Bals, S., Vanmaekelbergh, D., & de Mello Donega, C. (2017) · Journal of the American Chemical Society · doi:10.1021/jacs.6b13079 · Cited by 732
Strongly emissive perovskite nanocrystal inks for high-voltage solar cells
Akkerman, Q. A., Gandini, M., Di Stasio, F., Rastogi, P., Palazon, F., Bertoni, G., Ball, J. M., Prato, M., Petrozza, A., & Manna, L. (2016) · Nature Energy · doi:10.1038/nenergy.2016.194 · Cited by 721
Metadata
- Authors
- Sun, S., Yuan, D., Xu, Y., Wang, A., & Deng, Z.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-02-19
- Volume
- 10
- Issue
- 3
- Pages
- 3648-3657
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W2282847134
- Cited by
- 1,073
- References
- 1
- FWCI
- 64.49
- Type
- journal article
- Language
- en
- Open access
- closed
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- Sun, S., Yuan, D., Xu, Y., Wang, A., & Deng, Z. (2016). Ligand-Mediated Synthesis of Shape-Controlled Cesium Lead Halide Perovskite Nanocrystals via Reprecipitation Process at Room Temperature. ACS Nano. https://doi.org/10.1021/acsnano.5b08193
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