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Hybrid Perovskite/Perovskite Heterojunction Solar Cells
Open accessAbstract
Recently developed organic-inorganic hybrid perovskite solar cells combine low-cost fabrication and high power conversion efficiency. Advances in perovskite film optimization have led to an outstanding power conversion efficiency of more than 20%. Looking forward, shifting the focus toward new device architectures holds great potential to induce the next leap in device performance. Here, we demonstrate a perovskite/perovskite heterojunction solar cell. We developed a facile solution-based cation infiltration process to deposit layered perovskite (LPK) structures onto methylammonium lead iodide (MAPI) films. Grazing-incidence wide-angle X-ray scattering experiments were performed to gain insights into the crystallite orientation and the formation process of the perovskite bilayer. Our results show that the self-assembly of the LPK layer on top of an intact MAPI layer is accompanied by a reorganization of the perovskite interface. This leads to an enhancement of the open-circuit voltage and power conversion efficiency due to reduced recombination losses, as well as improved moisture stability in the resulting photovoltaic devices.
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Stranks, S. D., Eperon, G. E., Grancini, G., Menelaou, C., Alcocer, M. J. P., Leijtens, T., Herz, L. M., Petrozza, A., & Snaith, H. J. (2013) · Science · doi:10.1126/science.1243982 · Cited by 10,413
Solvent engineering for high-performance inorganic–organic hybrid perovskite solar cells
Jeon, N. J., Noh, J. H., Kim, Y. C., Yang, W. S., Ryu, S., & Seok, S. I. (2014) · Nature Materials · doi:10.1038/nmat4014 · Cited by 6,723
Cited by
Li, X., Hoffman, J. M., & Kanatzidis, M. G. (2021) · Chemical Reviews · doi:10.1021/acs.chemrev.0c01006 · Cited by 1,085
2D Ruddlesden–Popper Perovskites for Optoelectronics
Chen, Y., Sun, Y., Peng, J., Tang, J., Zheng, K., & Liang, Z. (2018) · Advanced Materials · doi:10.1002/adma.201703487 · Cited by 892
Present status and future prospects of perovskite photovoltaics
Snaith, H. J. (2018) · Nature Materials · doi:10.1038/s41563-018-0071-z · Cited by 803
Synthetic Approaches for Halide Perovskite Thin Films
Dunlap-Shohl, W. A., Zhou, Y., Padture, N. P., & Mitzi, D. B. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00318 · Cited by 631
Interfacial Residual Stress Relaxation in Perovskite Solar Cells with Improved Stability
Wang, H., Zhu, C., Liu, L., Ma, S., Liu, P., Wu, J., Shi, C., Du, Q., Hao, Y., Xiang, S., et al. (2019) · Advanced Materials · doi:10.1002/adma.201904408 · Cited by 499
Metadata
- Authors
- Hu, Y., Schlipf, J., Wussler, M., Petrus, M. L., Jaegermann, W., Bein, T., Müller-Buschbaum, P., & Docampo, P.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-06-03
- Volume
- 10
- Issue
- 6
- Pages
- 5999-6007
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W2402631077
- Cited by
- 345
- References
- 2
- FWCI
- 16.01
- Type
- journal article
- Language
- en
- Open access
- green
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- Hu, Y., Schlipf, J., Wussler, M., Petrus, M. L., Jaegermann, W., Bein, T., Müller-Buschbaum, P., & Docampo, P. (2016). Hybrid Perovskite/Perovskite Heterojunction Solar Cells. ACS Nano. https://doi.org/10.1021/acsnano.6b01535
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