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Cited by 203

The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.

Hydrogen-like Wannier–Mott Excitons in Single Crystal of Methylammonium Lead Bromide Perovskite

Tilchin, Jenya, Dirin, Dmitry N., Maikov, Georgy I., Sashchiuk, Aldona, Kovalenko, Maksym V., Lifshitz, Efrat·2016·ACS Nano

Abstract

A thorough investigation of exciton properties in bulk CH3NH3PbBr3 perovskite single crystals was carried out by recording the reflectance, steady-state and transient photoluminescence spectra of submicron volumes across the crystal. The study included an examination of the spectra profiles at various temperatures and laser excitation fluencies. The results resolved the first and second hydrogen-like Wannier-Mott exciton transitions at low temperatures, from which the ground-state exciton's binding energy of 15.33 meV and Bohr radius of ∼4.38 nm were derived. Furthermore, the photoluminescence temperature dependence suggested dominance of delayed exciton emission at elevated temperatures, originating from detrapping of carriers from shallow traps or/and from retrapping of electron-hole pairs into exciton states. The study revealed knowledge about several currently controversial issues that have an impact on functionality of perovskite materials in optoelectronic devices.

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Crossref · 10.1021/acsnano.6b02734

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Metadata

Authors
Tilchin, J., Dirin, D. N., Maikov, G. I., Sashchiuk, A., Kovalenko, M. V., & Lifshitz, E.
Venue
ACS Nano
Published
2016-06-06
Volume
10
Issue
6
Pages
6363-6371
ISSN
  • 1936-0851 (ISSN-L)
  • 1936-086X
OpenAlex
W2419272039
Cited by
203
References
3
FWCI
12.35
Type
journal article
Language
en
Open access
closed

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