Liquid Phase Exfoliated MoS2 Nanosheets Percolated with Carbon Nanotubes for High Volumetric/Areal Capacity Sodium-Ion Batteries

Liu, Yuping; He, Xiaoyun; Hanlon, Damien; Harvey, Andrew; Coleman, Jonathan N.; Li, Yanguang

doi:10.1021/acsnano.6b04577

Cited by 285Advancements in Battery MaterialsSupercapacitor Materials and FabricationMXene and MAX Phase Materials

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Liquid Phase Exfoliated MoS2 Nanosheets Percolated with Carbon Nanotubes for High Volumetric/Areal Capacity Sodium-Ion Batteries

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Liu, Yuping, He, Xiaoyun, Hanlon, Damien, Harvey, Andrew, Coleman, Jonathan N., Li, Yanguang·2016·ACS Nano

DOI 10.1021/acsnano.6b04577

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Abstract

The search for high-capacity, low-cost electrode materials for sodium-ion batteries is a significant challenge in energy research. Among the many potential candidates, layered compounds such as MoS2 have attracted increasing attention. However, such materials have not yet fulfilled their true potential. Here, we show that networks of liquid phase exfoliated MoS2 nanosheets, reinforced with 20 wt % single-wall carbon nanotubes (SWNTs), can be formed into sodium-ion battery electrodes with large gravimetric, volumetric, and areal capacity. The MoS2/SWNT composite films are highly porous, electrically conductive, and mechanically robust due to its percolating carbon nanotube network. When directly employed as the working electrode, they exhibit a specific capacity of >400 mAh/g and volumetric capacity of ∼650 mAh/cm(3). Their mechanical stability allows them to be processed into free-standing films with tunable thickness up to ∼100 μm, corresponding to an areal loading of 15 mg/cm(2). Their high electrical conductivity allows the high volumetric capacity to be retained, even at high thickness, resulting in state-of-the-art areal capacities of >4.0 mAh/cm(2). Such values are competitive with their lithium-ion counterparts.

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The lower electrochemical active surface areas and higher charge-transfer resistances of the two catalysts without net-like structure are attributed to agglomeration of MoS2 nanosheets and absence of conductive networks.
“the lower electrochemical active surface areas (Fig. 5i) and higher charge-transfer resistances (Fig. S9) of the two kinds of above catalyst without net-like structure are attributed to the agglomeration of MoS2 nanosheets and absence of conductive networks [62].”
From Defect-induced growth of MoS2 nanosheets on selectively etched SiC nanowires aerogel for efficient electrocatalytic hydrogen evolution (2025) · cites this paper as [62]

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Authors: Liu, Y., He, X., Hanlon, D., Harvey, A., Coleman, J. N., & Li, Y.
Affiliations: Soochow University (CN)
Trinity College Dublin (IE)
Corresponding author: Coleman, Jonathan N.
Li, Yanguang
ORCID: Liu, Yuping
He, Xiaoyun
Harvey, Andrew
Coleman, Jonathan N.
Li, Yanguang
Venue: ACS Nano
Publisher: American Chemical Society (ACS)
Published: 2016-08-23
Volume: 10
Issue: 9
Pages: 8821-8828
ISSN: 1936-0851 (ISSN-L)
1936-086X
DOI: 10.1021/acsnano.6b04577
OpenAlex: W2513234746
Cited by: 285
References: 53
Citations by year: 2026: 7 · 2025: 10 · 2024: 19 · 2023: 16 · 2022: 21 · 2021: 27 · 2020: 42 · 2019: 55 · 2018: 54 · 2017: 34
FWCI: 21.96
Type: journal article
Language: en
Open access: green
hdl.handle.net
Licence: cc-by-nc-sa
Locations: ACS Nano (publishedVersion)
PubMed (publishedVersion)
Trinity's Access to Research Output (TARA) (Trinity College Dublin) (submittedVersion, cc-by-nc-sa)
Funders: European Research Council (604391)
Science Foundation Ireland (11/PI/1087, SFI/12/RC/2278)
Natural Science Foundation of Jiangsu Province (BK20140302, SBK2015010320)
National Natural Science Foundation of China (51472173, 51522208)
Collaborative Innovation Center of Suzhou Nano Science and Technology
Priority Academic Program Development of Jiangsu Higher Education Institutions
Topics: Physical Sciences › Engineering › Electrical and Electronic Engineering › Advancements in Battery Materials
Physical Sciences › Materials Science › Electronic, Optical and Magnetic Materials › Supercapacitor Materials and Fabrication
Physical Sciences › Materials Science › Materials Chemistry › MXene and MAX Phase Materials
Keywords: sodium-ion batteries, MoS2 nanosheets, liquid-phase exfoliation, single-walled carbon nanotubes, volumetric capacity, areal capacity, gravimetric capacity, free-standing films, transition metal dichalcogenides

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Liquid Phase Exfoliated MoS2 Nanosheets Percolated with Carbon Nanotubes for High Volumetric/Areal Capacity Sodium-Ion Batteries

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