The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Polyphenol-Assisted Exfoliation of Transition Metal Dichalcogenides into Nanosheets as Photothermal Nanocarriers for Enhanced Antibiofilm Activity
Abstract
Transition metal dichalcogenide (TMD) nanosheets have evoked enormous research enthusiasm and have shown increased potentials in the biomedical field. However, a great challenge lies in high-throughput, large-scale, and eco-friendly preparation of TMD nanosheet dispersions with high quality. Herein, we report a universal polyphenol-assisted strategy to facilely exfoliate various TMDs into monolayer or few-layer nanosheets. By optimizing the exfoliation condition of molybdenum disulfide (MoS 2 ), the yield and concentration of as-exfoliated nanosheets are up to 60.5% and 1.21 mg/mL, respectively. This is the most efficient aqueous exfoliation method at present and is versatile for the choices of polyphenols and TMD nanomaterials. The as-exfoliated MoS 2 nanosheets possess superior biomedical stability as nanocarriers to load antibiotic drugs. They show a high photothermal conversion effect and thus induce a synergetic effect of chemotherapy and photothermal therapy to harvest enhanced antibiofilm activity under near-infrared (NIR) light. All these results offer an appealing strategy toward the synthesis and application of ultrathin TMD nanosheets, with great implications for their development.
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Cites
Mussel-inspired surface chemistry for multifunctional coatings
Lee, H., Dellatore, S. M., Miller, W. M., & Messersmith, P. B. (2007) · Science · doi:10.1126/science.1147241 · Cited by 10,965
Biofilms: an emergent form of bacterial life
Flemming, H.-C., Wingender, J., Szewzyk, U., Steinberg, P., Rice, S. A., & Kjelleberg, S. (2016) · Nature Reviews Microbiology · doi:10.1038/nrmicro.2016.94 · Cited by 5,979
High yield exfoliation of two-dimensional chalcogenides using sodium naphthalenide
Zheng, J., Zhang, H., Dong, S., Liu, Y., Tai Nai, C., Suk Shin, H., Young Jeong, H., Liu, B., & Ping Loh, K. (2014) · Nature Communications · doi:10.1038/ncomms3995 · Cited by 787
Cited by
Emerging photothermal-derived multimodal synergistic therapy in combating bacterial infections
Huo, J., Jia, Q., Huang, H., Zhang, J., Li, P., Dong, X., & Huang, W. (2021) · Chemical Society Reviews · doi:10.1039/d1cs00074h · Cited by 847
Mussel-inspired hydrogels: From design principles to promising applications
Zhang, C., Wu, B., Zhou, Y., Zhou, F., Liu, W., & Wang, Z. (2020) · Chemical Society Reviews · doi:10.1039/c9cs00849g · Cited by 653
Self-citationZhang, C., Zhou, Y., Han, H., Zheng, H., Xu, W., & Wang, Z. (2021) · ACS Nano · doi:10.1021/acsnano.0c09577 · Cited by 316
Self-citationQiu, D., Zheng, C., Zeng, Y., Wu, L., Huang, C., Ran, Y., Ding, Y., Shi, J., Cai, X., & Pan, Y. (2023) · Chemical Engineering Journal · doi:10.1016/j.cej.2023.147217 · Cited by 40
Metadata
- Authors
- Zhang, C., Hu, D.-F., Xu, J.-W., Ma, M.-Q., Xing, H., Yao, K., Ji, J., & Xu, Z.-K.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-12-03
- Volume
- 12
- Issue
- 12
- Pages
- 12347-12356
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W2903236462
- Cited by
- 197
- References
- 3
- FWCI
- 6.04
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhang, C., Hu, D.-F., Xu, J.-W., Ma, M.-Q., Xing, H., Yao, K., Ji, J., & Xu, Z.-K. (2018). Polyphenol-Assisted Exfoliation of Transition Metal Dichalcogenides into Nanosheets as Photothermal Nanocarriers for Enhanced Antibiofilm Activity. ACS Nano. https://doi.org/10.1021/acsnano.8b06321
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