The DOI matches its Crossref record; 38 of the 38 references it cites were found in a registry or an index.
Cathode Interfacial Layer Formation via in Situ Electrochemically Charging in Aqueous Zinc-Ion Battery
Abstract
The issue of material dissolution is common in aqueous batteries, leading to serious performance deterioration. However, it is difficult to be solved so far. In this study, a single component cathode solid electrolyte interface (SEI) layer (CaSO 4 ·2H 2 O) is observed via in situ electrochemically charging process, as demonstrated in a Ca 2 MnO 4 cathode for an aqueous zinc-ion battery. Density functional theory calculation confirms its electronic insulation and ionic conductor properties, indicating that it is an appropriate SEI film. The material dissolution seems to be effectively suppressed by the presence of the SEI layer on the cathode side. Meanwhile, this in situ formed interface layer is advantageous for lowering impedance, ameliorating interface, and reducing activation energy. As a result, significantly superior rate performance and cycle stability are exhibited. The observation of a protective SEI layer in an aqueous system may provide an insight into the development of high stability aqueous batteries.
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Cites
“Water-in-salt” electrolyte enables high-voltage aqueous lithium-ion chemistries
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Kundu, D., Adams, B. D., Duffort, V., Vajargah, S. H., & Nazar, L. F. (2016) · Nature Energy · doi:10.1038/nenergy.2016.119 · Cited by 3,124
Reversible aqueous zinc/manganese oxide energy storage from conversion reactions
Pan, H., Shao, Y., Yan, P., Cheng, Y., Han, K. S., Nie, Z., Wang, C., Yang, J., Li, X., Bhattacharya, P., et al. (2016) · Nature Energy · doi:10.1038/nenergy.2016.39 · Cited by 3,066
Issues and opportunities facing aqueous zinc-ion batteries
Tang, B., Shan, L., Liang, S., & Zhou, J. (2019) · Energy & Environmental Science · doi:10.1039/c9ee02526j · Cited by 2,182
Self-citationEnergetic Zinc Ion Chemistry: The Rechargeable Zinc Ion Battery
Xu, C., Li, B., Du, H., & Kang, F. (2012) · Angewandte Chemie International Edition · doi:10.1002/anie.201106307 · Cited by 2,055
Rechargeable aqueous zinc-manganese dioxide batteries with high energy and power densities
Zhang, N., Cheng, F., Liu, J., Wang, L., Long, X., Liu, X., Li, F., & Chen, J. (2017) · Nature Communications · doi:10.1038/s41467-017-00467-x · Cited by 1,796
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Rechargeable Aqueous Zn–V2O5 Battery with High Energy Density and Long Cycle Life
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Cited by
Advances and Perspectives of Cathode Storage Chemistry in Aqueous Zinc-Ion Batteries
Wang, X., Zhang, Z., Xi, B., Chen, W., Jia, Y., Feng, J., & Xiong, S. (2021) · ACS Nano · doi:10.1021/acsnano.1c01389 · Cited by 531
Zhou, M., Chen, Y., Fang, G., & Liang, S. (2022) · Energy Storage Materials · doi:10.1016/j.ensm.2021.12.011 · Cited by 316
Self-citationZheng, J., Pan, X., Huang, X., Xiong, D., Shang, Y., Li, X., Wang, N., Lau, W.-M., & Yang, H. Y. (2020) · Chemical Engineering Journal · doi:10.1016/j.cej.2020.125197 · Cited by 240
Metadata
- Authors
- Guo, S., Liang, S., Zhang, B., Fang, G., Ma, D., & Zhou, J.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2019-11-07
- Volume
- 13
- Issue
- 11
- Pages
- 13456-13464
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W2982822415
- Cited by
- 264
- References
- 38
- FWCI
- 11.28
- Type
- journal article
- Language
- en
- Open access
- closed
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- Guo, S., Liang, S., Zhang, B., Fang, G., Ma, D., & Zhou, J. (2019). Cathode Interfacial Layer Formation via in Situ Electrochemically Charging in Aqueous Zinc-Ion Battery. ACS Nano. https://doi.org/10.1021/acsnano.9b07042
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