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Cs2AgInCl6 Double Perovskite Single Crystals: Parity Forbidden Transitions and Their Application For Sensitive and Fast UV Photodetectors
Abstract
Double perovskite Cs 2 AgInCl 6 is newly reported as a stable and environmentally friendly alternative to lead halide perovskites. However, the fundamental properties of this material remain unexplored. Here, we first produced high-quality Cs 2 AgInCl 6 single crystals (SCs) with a low trap density of 8.6 × 10 8 cm –3, even lower than the value reported in the best lead halide perovskite SCs. Through systematical optical and electronic characterization, we experimentally verified the existence of the proposed parity-forbidden transition in Cs 2 AgInCl 6 and identified the role of oxygen in controlling its optical properties. Furthermore, sensitive (dectivity of ∼10 12 Jones), fast (3 dB bandwidth of 1035 Hz), and stable UV photodetectors were fabricated based on our Cs 2 AgInCl 6 SCs, showcasing their advantages for optoelectronic applications.
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Stranks, S. D., Eperon, G. E., Grancini, G., Menelaou, C., Alcocer, M. J. P., Leijtens, T., Herz, L. M., Petrozza, A., & Snaith, H. J. (2013) · Science · doi:10.1126/science.1243982 · Cited by 10,413
Lead halide perovskite nanowire lasers with low lasing thresholds and high quality factors
Zhu, H., Fu, Y., Meng, F., Wu, X., Gong, Z., Ding, Q., Gustafsson, M. V., Trinh, M. T., Jin, S., & Zhu, X.-Y. (2015) · Nature Materials · doi:10.1038/nmat4271 · Cited by 2,836
Cited by
Colloidal Synthesis of Double Perovskite Cs2AgInCl6 and Mn-Doped Cs2AgInCl6 Nanocrystals
Locardi, F., Cirignano, M., Baranov, D., Dang, Z., Prato, M., Drago, F., Ferretti, M., Pinchetti, V., Fanciulli, M., Brovelli, S., et al. (2018) · Journal of the American Chemical Society · doi:10.1021/jacs.8b07983 · Cited by 578
Rational Design of Halide Double Perovskites for Optoelectronic Applications
Zhao, X.-G., Yang, D., Ren, J.-C., Sun, Y., Xiao, Z., & Zhang, L. (2018) · Joule · doi:10.1016/j.joule.2018.06.017 · Cited by 508
Bi3+‐Er3+ and Bi3+‐Yb3+ Codoped Cs2AgInCl6 Double Perovskite Near‐Infrared Emitters
Arfin, H., Kaur, J., Sheikh, T., Chakraborty, S., & Nag, A. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.202002721 · Cited by 359
Structural and Functional Diversity in Lead‐Free Halide Perovskite Materials
Ning, W., & Gao, F. (2019) · Advanced Materials · doi:10.1002/adma.201900326 · Cited by 348
Emissive Bi-Doped Double Perovskite Cs2Ag1–xNaxInCl6 Nanocrystals
Locardi, F., Sartori, E., Buha, J., Zito, J., Prato, M., Pinchetti, V., Zaffalon, M. L., Ferretti, M., Brovelli, S., Infante, I., et al. (2019) · ACS Energy Letters · doi:10.1021/acsenergylett.9b01274 · Cited by 268
Metadata
- Authors
- Luo, J., Li, S., Wu, H., Zhou, Y., Li, Y., Liu, J., Li, J., Li, K., Yi, F., Niu, G., & Tang, J.
- Venue
- ACS Photonics
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-11-07
- Volume
- 5
- Issue
- 2
- Pages
- 398-405
- ISSN
- 2330-4022 (ISSN-L)
- OpenAlex
- W2767197417
- Cited by
- 442
- References
- 2
- FWCI
- 12.31
- Type
- journal article
- Language
- en
- Open access
- closed
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