The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Defective Carbon-Based Materials for the Electrochemical Synthesis of Hydrogen Peroxide
Open accessAbstract
Hydrogen peroxide (H 2 O 2 ), an important industrial chemical, is currently produced through an energy-intensive anthraquinone process that is limited to large-scale facilities. Small-scale decentralized electrochemical production of H 2 O 2 via a two-electron oxygen reduction reaction (ORR) offers unique opportunities for sanitization applications and the purification of drinking water. The development of inexpensive, efficient, and selective catalysts for this reaction remains a challenge. Herein, we examine two different porous carbon-based electrocatalysts and show that they exhibit high selectivity for H 2 O 2 under alkaline conditions. By rationally varying synthetic methods, we explore the effect of pore size on electrocatalytic performance. Furthermore, by means of density functional calculations, we point out the critical role of carbon defects. Our theory results show that the majority of defects in graphene are naturally selective for the two-electron reduction of O 2 to H 2 O 2, and we identify the types of defects with high activity.
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Cites
Origin of the Overpotential for Oxygen Reduction at a Fuel-Cell Cathode
Nørskov, J. K., Rossmeisl, J., Logadottir, A., Lindqvist, L., Kitchin, J. R., Bligaard, T., & Jónsson, H. (2004) · The Journal of Physical Chemistry B · doi:10.1021/jp047349j · Cited by 13,153
Self-citationAbild-Pedersen, F., Greeley, J., Studt, F., Rossmeisl, J., Munter, T. R., Moses, P. G., Skúlason, E., Bligaard, T., & Nørskov, J. K. (2007) · Physical Review Letters · doi:10.1103/physrevlett.99.016105 · Cited by 1,678
Self-citationTuning selectivity of electrochemical reactions by atomically dispersed platinum catalyst
Choi, C. H., Kim, M., Kwon, H. C., Cho, S. J., Yun, S., Kim, H.-T., Mayrhofer, K. J. J., Kim, H., & Choi, M. (2016) · Nature Communications · doi:10.1038/ncomms10922 · Cited by 849
Cited by
Highly selective oxygen reduction to hydrogen peroxide on transition metal single atom coordination
Jiang, K., Back, S., Akey, A. J., Xia, C., Hu, Y., Liang, W., Schaak, D., Stavitski, E., Nørskov, J. K., Siahrostami, S., et al. (2019) · Nature Communications · doi:10.1038/s41467-019-11992-2 · Cited by 820
Self-citationZnO As an Active and Selective Catalyst for Electrochemical Water Oxidation to Hydrogen Peroxide
Kelly, S. R., Shi, X., Back, S., Vallez, L., Park, S. Y., Siahrostami, S., Zheng, X., & Nørskov, J. K. (2019) · ACS Catalysis · doi:10.1021/acscatal.8b04873 · Cited by 298
Self-citationPulsed Laser in Liquids Made Nanomaterials for Catalysis
Forsythe, R. C., Cox, C. P., Wilsey, M. K., & Müller, A. M. (2021) · Chemical Reviews · doi:10.1021/acs.chemrev.0c01069 · Cited by 259
KOH-treated reduced graphene oxide: 100% selectivity for H2O2 electroproduction
Zhu, J., Xiao, X., Zheng, K., Li, F., Ma, G., Yao, H.-C., Wang, X., & Chen, Y. (2019) · Carbon · doi:10.1016/j.carbon.2019.07.009 · Cited by 111
Metadata
- Authors
- Chen, S., Chen, Z., Siahrostami, S., Kim, T. R., Nordlund, D., Sokaras, D., Nowak, S., To, J. W. F., Higgins, D., Sinclair, R., Nørskov, J. K., Jaramillo, T. F., & Bao, Z.
- Venue
- ACS Sustainable Chemistry & Engineering
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-11-14
- Volume
- 6
- Issue
- 1
- Pages
- 311-317
- ISSN
- 2168-0485 (ISSN-L)
- OpenAlex
- W2765517692
- Cited by
- 354
- References
- 3
- FWCI
- 5.48
- Type
- journal article
- Language
- en
- Open access
- green
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- Chen, S., Chen, Z., Siahrostami, S., Kim, T. R., Nordlund, D., Sokaras, D., Nowak, S., To, J. W. F., Higgins, D., Sinclair, R., Nørskov, J. K., Jaramillo, T. F., & Bao, Z. (2018). Defective Carbon-Based Materials for the Electrochemical Synthesis of Hydrogen Peroxide. ACS Sustainable Chemistry & Engineering. https://doi.org/10.1021/acssuschemeng.7b02517
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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