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Efficient Electrochemical N2 Reduction to NH3 on MoN Nanosheets Array under Ambient Conditions
Abstract
Electrochemical N 2 reduction reaction (NRR) under ambient conditions offers us an environmentally friendly route for artificial synthesis of NH 3 . However, up to now, few noble-metal-free electrocatalysts with satisfactory catalytic activities have been explored. In this Letter, we demonstrate that MoN nanosheets array on carbon cloth (MoN NA/CC) acts as a high-performance NRR electrocatalyst toward NH 3 electrosynthesis in 0.1 M HCl under ambient conditions. This catalyst achieves a large NH 3 yield of 3.01 × 10 –10 mo1 s –1 cm –2 and a Faradaic efficiency of 1.15% at −0.3 V vs reversible hydrogen electrode with strong electrochemical durability and selectivity. Density functional theory calculations reveal that MoN NA/CC catalyzes NRR via the Mars–van Krevelen mechanism.
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Kibsgaard, J., Chen, Z., Reinecke, B. N., & Jaramillo, T. F. (2012) · Nature Materials · doi:10.1038/nmat3439 · Cited by 3,234
Tian, J., Liu, Q., Asiri, A. M., & Sun, X. (2014) · Journal of the American Chemical Society · doi:10.1021/ja503372r · Cited by 2,373
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Cited by
Defect engineering in earth-abundant electrocatalysts for CO2 and N2 reduction
Wang, Q., Lei, Y., Wang, D., & Li, Y. (2019) · Energy & Environmental Science · doi:10.1039/c8ee03781g · Cited by 574
Comprehensive Understanding of the Thriving Ambient Electrochemical Nitrogen Reduction Reaction
Zhao, X., Hu, G., Chen, G., Zhang, H., Zhang, S., & Wang, H. (2021) · Advanced Materials · doi:10.1002/adma.202007650 · Cited by 503
Zhang, Y., Qiu, W., Ma, Y., Luo, Y., Tian, Z., Cui, G., Xie, F., Chen, L., Li, T., & Sun, X. (2018) · ACS Catalysis · doi:10.1021/acscatal.8b02311 · Cited by 293
Self-citationEnhancing Electrocatalytic N2 Reduction to NH3 by CeO2 Nanorod with Oxygen Vacancies
Xu, B., Xia, L., Zhou, F., Zhao, R., Chen, H., Wang, T., Zhou, Q., Liu, Q., Cui, G., Xiong, X., et al. (2019) · ACS Sustainable Chemistry & Engineering · doi:10.1021/acssuschemeng.8b05007 · Cited by 151
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Metadata
- Authors
- Zhang, L., Ji, X., Ren, X., Luo, Y., Shi, X., Asiri, A. M., Zheng, B., & Sun, X.
- Venue
- ACS Sustainable Chemistry & Engineering
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-07-13
- Volume
- 6
- Issue
- 8
- Pages
- 9550-9554
- ISSN
- 2168-0485 (ISSN-L)
- OpenAlex
- W2883974747
- Cited by
- 241
- References
- 2
- FWCI
- 8.82
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhang, L., Ji, X., Ren, X., Luo, Y., Shi, X., Asiri, A. M., Zheng, B., & Sun, X. (2018). Efficient Electrochemical N2 Reduction to NH3 on MoN Nanosheets Array under Ambient Conditions. ACS Sustainable Chemistry & Engineering. https://doi.org/10.1021/acssuschemeng.8b01438
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