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Solvothermal One-Step Synthesis of Ni–Al Layered Double Hydroxide/Carbon Nanotube/Reduced Graphene Oxide Sheet Ternary Nanocomposite with Ultrahigh Capacitance for Supercapacitors

Yang, Wanlu, Gao, Zan, Wang, Jun, Ma, Jing, Zhang, Milin, Liu, Lianhe·2013·ACS Applied Materials & Interfaces

Abstract

A Ni-Al layered double hydroxide (LDH), mutil-wall carbon nanotube (CNT), and reduced graphene oxide sheet (GNS) ternary nanocomposite electrode material has been developed by a facile one-step ethanol solvothermal method. The obtained LDH/CNT/GNS composite displayed a three-dimensional (3D) architecture with flowerlike Ni-Al LDH/CNT nanocrystallites gradually self-assembled on GNS nanosheets. GNS was used as building blocks to construct 3D nanostructure, and the LDH/CNT nanoflowers in turn separated the two-dimensional (2D) GNS sheets, which preserved the high surface area of GNSs. Furthermore, the generated porous networks with a narrow pore size distribution in the LDH/CNT/GNS composite were also demonstrated by the N2 adsorption/desorption experiment. Such morphology would be favorable to improve the mass transfer and electrochemical action of the electrode. As supercapacitor electrode material, the LDH/CNT/GNS hybrid exhibited excellent electrochemical performance, including ultrahigh specific capacitance (1562 F/g at 5 mA/cm(2)), excellent rate capability, and long-term cycling performance, which could be a promising energy storage/conversion material for supercapacitor application.

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Metadata

Authors
Yang, W., Gao, Z., Wang, J., Ma, J., Zhang, M., & Liu, L.
Venue
ACS Applied Materials & Interfaces
Published
2013-06-05
Volume
5
Issue
12
Pages
5443-5454
ISSN
  • 1944-8244 (ISSN-L)
  • 1944-8252
OpenAlex
W2005963921
Cited by
272
References
2
FWCI
9.65
Type
journal article
Language
en
Open access
closed

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CoChat. (2026). Citation check: Solvothermal One-Step Synthesis of Ni–Al Layered Double Hydroxide/Carbon Nanotube/Reduced Graphene Oxide Sheet Ternary Nanocomposite with Ultrahigh Capacitance for Supercapacitors. https://app.cochat.ai/papers/10.1021/am4003843
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Yang, W., Gao, Z., Wang, J., Ma, J., Zhang, M., & Liu, L. (2013). Solvothermal One-Step Synthesis of Ni–Al Layered Double Hydroxide/Carbon Nanotube/Reduced Graphene Oxide Sheet Ternary Nanocomposite with Ultrahigh Capacitance for Supercapacitors. ACS Applied Materials & Interfaces. https://doi.org/10.1021/am4003843

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