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Understanding Water Permeation in Graphene Oxide Membranes
Open accessAbstract
Water transport through graphene-derived membranes has gained much interest recently due to its promising potential in filtration and separation applications. In this work, we explore water permeation in graphene oxide membranes using atomistic simulations and theoretical analysis, by considering flow through the interlayer gallery, expanded channels such as wrinkles of interedge spaces, and pores within the sheet. We find that, although flow enhancement can be established by nanoconfinement, fast water transport through pristine graphene channels is prohibited by a prominent side-pinning effect from capillaries formed within oxidized regions. We then discuss several flow enhancement mechanisms through the porous microstructures of graphene oxide membranes. These understandings are integrated into a complete picture to understand water permeation through the layer-by-layer and porous microstructure and can guide rational design of functional membranes for energy and environmental applications.
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Cites
Fast Parallel Algorithms for Short-Range Molecular Dynamics
Plimpton, S. (1995) · Journal of Computational Physics · doi:10.1006/jcph.1995.1039 · Cited by 44,721
The chemistry of graphene oxide
Dreyer, D. R., Park, S., Bielawski, C. W., & Ruoff, R. S. (2010) · Chem. Soc. Rev. · doi:10.1039/b917103g · Cited by 11,653
Cited by
High-Flux Graphene Oxide Nanofiltration Membrane Intercalated by Carbon Nanotubes
Han, Y., Jiang, Y., & Gao, C. (2015) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.5b00986 · Cited by 532
Graphene membranes for water desalination
Homaeigohar, S., & Elbahri, M. (2017) · NPG Asia Materials · doi:10.1038/am.2017.135 · Cited by 444
Graphene-Based Membranes for Molecular Separation
Huang, L., Zhang, M., Li, C., & Shi, G. (2015) · The Journal of Physical Chemistry Letters · doi:10.1021/acs.jpclett.5b00914 · Cited by 391
Anand, A., Unnikrishnan, B., Mao, J.-Y., Lin, H.-J., & Huang, C.-C. (2018) · Desalination · doi:10.1016/j.desal.2017.12.012 · Cited by 339
2D Laminar Membranes for Selective Water and Ion Transport
Kang, Y., Xia, Y., Wang, H., & Zhang, X. (2019) · Advanced Functional Materials · doi:10.1002/adfm.201902014 · Cited by 325
Metadata
- Authors
- Wei, N., Peng, X., & Xu, Z.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-04-10
- Volume
- 6
- Issue
- 8
- Pages
- 5877-5883
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W1987709643
- Cited by
- 487
- References
- 2
- FWCI
- 20.03
- Type
- journal article
- Language
- en
- Open access
- green
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- Wei, N., Peng, X., & Xu, Z. (2014). Understanding Water Permeation in Graphene Oxide Membranes. ACS Applied Materials & Interfaces. https://doi.org/10.1021/am500777b
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
