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The Development of L2X2RuCHR Olefin Metathesis Catalysts: An Organometallic Success Story
Abstract
In recent years, the olefin metathesis reaction has attracted widespread attention as a versatile carbon-carbon bond-forming method. Many new applications have become possible because of major advances in catalyst design. State-of-the-art ruthenium catalysts are not only highly active but also compatible with most functional groups and easy to use. This Account traces the ideas and discoveries that were instrumental in the development of these catalysts, with particular emphasis on (PCy3)2Cl2Ru=CHPh and its derivatives. The discussion includes an analysis of trends in catalyst activity, a description of catalysts coordinated with N-heterocyclic carbene ligands, and an overview of ongoing work to improve the activity, stability, and selectivity of this family of L2X2Ru=CHR complexes.
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The development of functional group tolerant ROMP catalysts
Grubbs, R. H. (1994) · Journal of Macromolecular Science, Part A · doi:10.1080/10601329408545884 · Cited by 95
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Cited by
Heterocyclic Carbenes: Synthesis and Coordination Chemistry
Hahn, F. E., & Jahnke, M. C. (2008) · Angewandte Chemie International Edition · doi:10.1002/anie.200703883 · Cited by 2,775
Organocatalytic Ring-Opening Polymerization
Kamber, N. E., Jeong, W., Waymouth, R. M., Pratt, R. C., Lohmeijer, B. G. G., & Hedrick, J. L. (2007) · Chemical Reviews · doi:10.1021/cr068415b · Cited by 1,489
Vegetable oil-based polymeric materials: synthesis, properties, and applications
Xia, Y., & Larock, R. C. (2010) · Green Chemistry · doi:10.1039/c0gc00264j · Cited by 864
Macromolecular architectures by living and controlled/living polymerizations
Hadjichristidis, N., Iatrou, H., Pitsikalis, M., & Mays, J. (2006) · Progress in Polymer Science · doi:10.1016/j.progpolymsci.2006.07.002 · Cited by 642
Decomposition of a Key Intermediate in Ruthenium-Catalyzed Olefin Metathesis Reactions
Hong, S. H., Day, M. W., & Grubbs, R. H. (2004) · Journal of the American Chemical Society · doi:10.1021/ja0488380 · Cited by 414
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Metadata
- Authors
- Trnka, T. M., & Grubbs, R. H.
- Venue
- Accounts of Chemical Research
- Publisher
- American Chemical Society (ACS)
- Published
- 2000-11-04
- Volume
- 34
- Issue
- 1
- Pages
- 18-29
- ISSN
- 0001-4842 (ISSN-L)
- 1520-4898
- OpenAlex
- W2116741024
- Cited by
- 3,561
- References
- 1
- FWCI
- 132.74
- Type
- journal article
- Language
- en
- Open access
- closed
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- Trnka, T. M., & Grubbs, R. H. (2001). The Development of L2X2RuCHR Olefin Metathesis Catalysts: An Organometallic Success Story. Accounts of Chemical Research. https://doi.org/10.1021/ar000114f
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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