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Energy Dissipation in Multichromophoric Single Dendrimers
Abstract
Single-molecule spectroscopy of well-chosen dendritic multichromophoric systems allows investigation of fundamental photophysical processes such as energy or electron transfer in much greater detail than the respective ensemble measurements. In dendrimers with multiple chromophores, energy hopping and transfer to the chromophore with the energetically lowest S(1) state was observed. If more than one chromophore is in an excited state in one molecule, annihilation, either singlet-triplet or singlet-singlet, can occur. In the latter case, a higher singlet state is populated opening new deactivation pathways. In the presence of an electron donor, reversible electron transfer could be observed, and the rate constants of forward and backward electron transfer were established. The value of these rate constants fluctuates time-correlated with the rotational motion of the dendrimer arms and the mobility of the embedding matrix.
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Logical computation using algorithmic self-assembly of DNA triple-crossover molecules
Mao, C., LaBean, T. H., Reif, J. H., & Seeman, N. C. (2000) · Nature · doi:10.1038/35035038 · Cited by 779
Single chain spectroscopy of conformational dependence of conjugated polymer photophysics
Huser, T., Yan, M., & Rothberg, L. J. (2000) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.97.21.11187 · Cited by 322
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Imaging molecular interactions in living cells by FRET microscopy
Jares-Erijman, E. A., & Jovin, T. M. (2006) · Current Opinion in Chemical Biology · doi:10.1016/j.cbpa.2006.08.021 · Cited by 313
Collective fluorescence switching of counterion-assembled dyes in polymer nanoparticles
Reisch, A., Didier, P., Richert, L., Oncul, S., Arntz, Y., Mély, Y., & Klymchenko, A. S. (2014) · Nature Communications · doi:10.1038/ncomms5089 · Cited by 226
A “breathing” dendritic molecule—conformational fluctuation induced by external stimuli
Zeng, Y., Li, P., Liu, X., Yu, T., Chen, J., Yang, G., & Li, Y. (2014) · Polym. Chem. · doi:10.1039/c4py00714j · Cited by 22
Metadata
- Authors
- De Schryver, F. C., Vosch, T., Cotlet, M., Van der Auweraer, M., Müllen, K., & Hofkens, J.
- Venue
- Accounts of Chemical Research
- Publisher
- American Chemical Society (ACS)
- Published
- 2004-12-07
- Volume
- 38
- Issue
- 7
- Pages
- 514-522
- ISSN
- 0001-4842 (ISSN-L)
- 1520-4898
- OpenAlex
- W2120320561
- Cited by
- 272
- References
- 2
- FWCI
- 13.36
- Type
- journal article
- Language
- en
- Open access
- closed
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- De Schryver, F. C., Vosch, T., Cotlet, M., Van der Auweraer, M., Müllen, K., & Hofkens, J. (2005). Energy Dissipation in Multichromophoric Single Dendrimers. Accounts of Chemical Research. https://doi.org/10.1021/ar040126r
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