The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Catalyst Morphology and Dissolution Kinetics of Self-Healing Polymers
Abstract
The role of the crystal morphology and dissolution kinetics of Grubbs' catalyst on self-healing capability is examined. Self-healing polymers require complete coverage of the crack plane with polymerized healing agent for optimal recovery of mechanical integrity. Lack of catalyst leads to incomplete coverage, partial polymerization, and poor mechanical recovery. Catalyst availability is determined by the competing rates of dissolution of the catalyst and polymerization of the healing agent. First-generation Grubbs' catalyst exists in at least two crystal polymorphs, each with a distinct crystal shape, thermal stability, and dissolution kinetics. The more rapidly dissolving polymorph shows superior healing efficiency when used as the initiator in a self-healing epoxy material based on ring-opening metathesis polymerization of dicyclopentadiene.
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Cites
A chiroselective peptide replicator
Saghatelian, A., Yokobayashi, Y., Soltani, K., & Ghadiri, M. R. (2001) · Nature · doi:10.1038/35057238 · Cited by 310
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Self-healing materials with microvascular networks
Toohey, K. S., Sottos, N. R., Lewis, J. A., Moore, J. S., & White, S. R. (2007) · Nature Materials · doi:10.1038/nmat1934 · Cited by 1,633
Self-citationMechanically-Induced Chemical Changes in Polymeric Materials
Caruso, M. M., Davis, D. A., Shen, Q., Odom, S. A., Sottos, N. R., White, S. R., & Moore, J. S. (2009) · Chemical Reviews · doi:10.1021/cr9001353 · Cited by 1,372
Self-citationZhu, D. Y., Rong, M. Z., & Zhang, M. Q. (2015) · Progress in Polymer Science · doi:10.1016/j.progpolymsci.2015.07.002 · Cited by 631
Multifunctional Energy Storage and Conversion Devices
Huang, Y., Zhu, M., Huang, Y., Pei, Z., Li, H., Wang, Z., Xue, Q., & Zhi, C. (2016) · Advanced Materials · doi:10.1002/adma.201601928 · Cited by 544
Embedded Shape‐Memory Alloy Wires for Improved Performance of Self‐Healing Polymers
Kirkby, E. L., Rule, J. D., Michaud, V. J., Sottos, N. R., White, S. R., & Månson, J. E. (2008) · Advanced Functional Materials · doi:10.1002/adfm.200701208 · Cited by 207
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Metadata
- Authors
- Jones, A. S., Rule, J. D., Moore, J. S., White, S. R., & Sottos, N. R.
- Venue
- Chemistry of Materials
- Publisher
- American Chemical Society (ACS)
- Published
- 2006-02-03
- Volume
- 18
- Issue
- 5
- Pages
- 1312-1317
- ISSN
- 0897-4756 (ISSN-L)
- 1520-5002
- OpenAlex
- W2067063229
- Cited by
- 210
- References
- 1
- FWCI
- 16.29
- Type
- journal article
- Language
- en
- Open access
- closed
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