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Synthesis and Lithium Storage Mechanism of Ultrafine MoO2 Nanorods
Abstract
Ultrafine MoO 2 nanorods with a diameter of ∼5 nm were successfully synthesized by a nanocasting method using mesoporous silica SBA-15 as hard template. This material demonstrates high reversible capacity, excellent cycling performance, and good rate capacity as an anode electrode material for Li ion batteries. The significant enhancement in the electrochemical Li storage performance in ultrafine MoO 2 nanorods is attributed to the nanorod structure with small diameter and efficient one-dimensional electron transport pathways. Moreover, density functional theory calculations were performed to elucidate the Li uptake/removal mechanism in the MoO 2 electrodes, which can help us understand the unique cycling behavior of MoO 2 material.
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Citations
Cites
Characterization of the porous structure of sba-15
Kruk, M., Jaroniec, M., Ko, C. H., & Ryoo, R. (2000) · Chemistry of Materials · doi:10.1021/cm000164e · Cited by 1,409
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Lu, Y., Yu, L., & Lou, X. W. (. (2018) · Chem · doi:10.1016/j.chempr.2018.01.003 · Cited by 783
Nanostructured Mo-based electrode materials for electrochemical energy storage
Hu, X., Zhang, W., Liu, X., Mei, Y., & Huang, Y. (2015) · Chemical Society Reviews · doi:10.1039/c4cs00350k · Cited by 711
Multi-scale computation methods: Their applications in lithium-ion battery research and development
Shi, S., Gao, J., Liu, Y., Zhao, Y., Wu, Q., Ju, W., Ouyang, C., & Xiao, R. (2016) · Chinese Physics B · doi:10.1088/1674-1056/25/1/018212 · Cited by 615
Self-citationZhao, Y., Wang, L. P., Sougrati, M. T., Feng, Z., Leconte, Y., Fisher, A., Srinivasan, M., & Xu, Z. (2017) · Advanced Energy Materials · doi:10.1002/aenm.201601424 · Cited by 586
Exploring Anomalous Charge Storage in Anode Materials for Next-Generation Li Rechargeable Batteries
Kim, H., Choi, W., Yoon, J., Um, J. H., Lee, W., Kim, J., Cabana, J., & Yoon, W.-S. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00618 · Cited by 527
Metadata
- Authors
- Guo, B., Fang, X., Li, B., Shi, Y., Ouyang, C., Hu, Y.-S., Wang, Z., Stucky, G. D., & Chen, L.
- Venue
- Chemistry of Materials
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-01-17
- Volume
- 24
- Issue
- 3
- Pages
- 457-463
- ISSN
- 0897-4756 (ISSN-L)
- 1520-5002
- OpenAlex
- W2312321370
- Cited by
- 242
- References
- 1
- FWCI
- 9.58
- Type
- journal article
- Language
- en
- Open access
- closed
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- Guo, B., Fang, X., Li, B., Shi, Y., Ouyang, C., Hu, Y.-S., Wang, Z., Stucky, G. D., & Chen, L. (2012). Synthesis and Lithium Storage Mechanism of Ultrafine MoO2 Nanorods. Chemistry of Materials. https://doi.org/10.1021/cm202459r
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