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MOF-Derived Hierarchically Porous Carbon with Exceptional Porosity and Hydrogen Storage Capacity
Abstract
Highly porous carbon has played an important role in tackling down the energy and environmental problems due to their attractive features such as high specific surface area (SSA), stability, and mass productivity. Especially, the desirable characteristics of the highly porous carbon such as lightweight, fast adsorption/desorption kinetics, and high SSA have attracted extensive attention in the “hydrogen storage” application which is a main bottleneck for the realization of on-board hydrogen fuel cell vehicles. We herein presented porous carbon with hierarchical pore structure derived from highly crystalline metal organic frameworks (denoted as MOF-derived carbon: MDC) without any carbon source and showed it as a promising hydrogen storage adsorbent. MDCs can be fabricated by a simple heat adjustment of MOFs without complicated process and environmental burden. The MDC displayed hierarchical pore structures with high ultramicroporosity, high SSA, and very high total pore volume. Due to its exceptional porosity, MDCs exhibited reversible H 2 storage capacities at certain conditions that were better than those of previously reported porous carbons and MOFs.
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Cites
Engineering carbon materials from the hydrothermal carbonization process of biomass
Hu, B., Wang, K., Wu, L., Yu, S., Antonietti, M., & Titirici, M. (2010) · Advanced Materials · doi:10.1002/adma.200902812 · Cited by 1,765
Metal–organic framework (MOF) aerogels with high micro- and macroporosity
Lohe, M. R., Rose, M., & Kaskel, S. (2009) · Chemical Communications · doi:10.1039/b910175f · Cited by 286
Cited by
Hou, J., Cao, C., Idrees, F., & Ma, X. (2015) · ACS Nano · doi:10.1021/nn506394r · Cited by 1,529
Sun, M.-H., Huang, S.-Z., Chen, L.-H., Li, Y., Yang, X.-Y., Yuan, Z.-Y., & Su, B.-L. (2016) · Chemical Society Reviews · doi:10.1039/c6cs00135a · Cited by 1,454
Xu, X., Cao, R., Jeong, S., & Cho, J. (2012) · Nano Letters · doi:10.1021/nl302618s · Cited by 914
Metal organic frameworks for electrochemical applications
Morozan, A., & Jaouen, F. (2012) · Energy & Environmental Science · doi:10.1039/c2ee22989g · Cited by 870
Graphene-based materials: Synthesis and gas sorption, storage and separation
Gadipelli, S., & Guo, Z. X. (2015) · Progress in Materials Science · doi:10.1016/j.pmatsci.2014.10.004 · Cited by 734
Metadata
- Authors
- Yang, S. J., Kim, T., Im, J. H., Kim, Y. S., Lee, K., Jung, H., & Park, C. R.
- Venue
- Chemistry of Materials
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-01-25
- Volume
- 24
- Issue
- 3
- Pages
- 464-470
- ISSN
- 0897-4756 (ISSN-L)
- 1520-5002
- OpenAlex
- W2061132599
- Cited by
- 749
- References
- 2
- FWCI
- 25.77
- Type
- journal article
- Language
- en
- Open access
- closed
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