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Hydrogen Storage Properties of Space-Confined NaAlH4 Nanoparticles in Ordered Mesoporous Silica
Abstract
A method that is used by space-confining NaAlH 4 into the as-synthesized ordered mesoporous silica (OMS) is presented in the present work. NaAlH 4 in the pores of OMS is obtained by impregnation and drying techniques. It has been found that the space-confined NaAlH 4 in the pores of OMS shows the lower temperature and faster kinetics for dehydrogenation than that of the pristine NaAlH 4 . Moreover, in the absence of a catalyst, the rehydrogenation in a dehydrogenated NaAlH 4 system with nanoscale particles and phases can be achieved even with the temperatures of 125−150 °C and the hydrogen pressures of 3.5−5.5 MPa. The physical limitation of the NaAlH 4 particles, as well as the resulting Al and NaH phases, to be nanoscale in size by the pores of OMS is believed to be responsible for these.
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Cites
Metal hydride materials for solid hydrogen storage: A review
SAKINTUNA, B., LAMARIDARKRIM, F., & HIRSCHER, M. (2007) · International Journal of Hydrogen Energy · doi:10.1016/j.ijhydene.2006.11.022 · Cited by 3,715
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Nanomaterials for renewable energy production and storage
Chen, X., Li, C., Grätzel, M., Kostecki, R., & Mao, S. S. (2012) · Chemical Society Reviews · doi:10.1039/c2cs35230c · Cited by 1,015
Yu, X., Tang, Z., Sun, D., Ouyang, L., & Zhu, M. (2017) · Progress in Materials Science · doi:10.1016/j.pmatsci.2017.03.001 · Cited by 716
Self-citationAdvanced carbon aerogels for energy applications
Biener, J., Stadermann, M., Suss, M., Worsley, M. A., Biener, M. M., Rose, K. A., & Baumann, T. F. (2011) · Energy & Environmental Science · doi:10.1039/c0ee00627k · Cited by 651
Hydrogen in magnesium: new perspectives toward functional stores
Aguey-Zinsou, K.-F., & Ares-Fernández, J.-R. (2010) · Energy & Environmental Science · doi:10.1039/b921645f · Cited by 447
Hydrogen Storage Materials for Mobile and Stationary Applications: Current State of the Art
Lai, Q., Paskevicius, M., Sheppard, D. A., Buckley, C. E., Thornton, A. W., Hill, M. R., Gu, Q., Mao, J., Huang, Z., Liu, H. K., et al. (2015) · ChemSusChem · doi:10.1002/cssc.201500231 · Cited by 414
Metadata
- Authors
- Zheng, S., Fang, F., Zhou, G., Chen, G., Ouyang, L., Zhu, M., & Sun, D.
- Venue
- Chemistry of Materials
- Publisher
- American Chemical Society (ACS)
- Published
- 2008-05-21
- Volume
- 20
- Issue
- 12
- Pages
- 3954-3958
- ISSN
- 0897-4756 (ISSN-L)
- 1520-5002
- OpenAlex
- W1970602067
- Cited by
- 195
- References
- 1
- FWCI
- 6.74
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Hydrogen Storage Properties of Space-Confined NaAlH4 Nanoparticles in Ordered Mesoporous Silica. https://app.cochat.ai/papers/10.1021/cm8002063
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- Zheng, S., Fang, F., Zhou, G., Chen, G., Ouyang, L., Zhu, M., & Sun, D. (2008). Hydrogen Storage Properties of Space-Confined NaAlH4 Nanoparticles in Ordered Mesoporous Silica. Chemistry of Materials. https://doi.org/10.1021/cm8002063
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